介质阻挡微等离子体转化CH4制低碳烃-化学工程专业论文.docxVIP

A simplified global chemical kinetic model according to methane concentration was proposed. The chemical kinetic model showed that the conversion of methane was an exponential function of the plasma energy for a low methane inlet concentration, and was a linear function of the input energy for a high methane inlet concentration. The chemical kinetic in different micro-DBD reactors was inveatigated. The reaults showed that a micro-DBD reactor with smaller discharge gap had high rate of production radicals and high energy efficiency. A nonlinear multiple regression analysis was appropriate for data regression and for the correlation of system variables with both the conversion of methane and product selectivity. KEYWORDS：micro-DBD, methane, hydrocarbon, reactor, kinetic 目 录 第一章 文献综述 1 HYPERLINK \l _bookmark0 1.1 引言 1 HYPERLINK \l _bookmark1 1.2 微等离子体技术 1 HYPERLINK \l _bookmark2 1.2.1 微等离子体技术定义 1 HYPERLINK \l _bookmark3 1.2.2 微等离子体技术的特点 2 HYPERLINK \l _bookmark4 1.2.3 微等离子体技术分类 2 HYPERLINK \l _bookmark5 1.2.4 微等离子体的产生及应用 2 HYPERLINK \l _bookmark6 1.3 等离子体技术转化 CH4 的研究进展 7 HYPERLINK \l _bookmark7 1.3.1 CH4 非氧化转化 7 HYPERLINK \l _bookmark8 CH4-CO2 重整 9 HYPERLINK \l _bookmark9 CH4-H2O 重整 11 HYPERLINK \l _bookmark10 1.3.4 CH4 部分氧化转化 12 HYPERLINK \l _bookmark11 1.4 DBD-微等离子体用于 CH4 转化的应用前景 13 HYPERLINK \l _bookmark12 1.5 论文工作的提出及论文内容 14 HYPERLINK \l _bookmark13 第二章 实验部分 15 HYPERLINK \l _bookmark14 2.1 介质阻挡微等离子体转化 CH4 机理 15 HYPERLINK \l _bookmark15 2.2 实验装置及反应流程 17 HYPERLINK \l _bookmark16 2.2.1 介质阻挡微等离子体反应器形式 17 HYPERLINK \l _bookmark17 2.2.2 介质阻挡微等离子体反应器尺寸 17 HYPERLINK \l _bookmark18 2.2.3 实验流程 18 HYPERLINK \l _bookmark19 2.3 实验原料 19 HYPERLINK \l _bookmark20 2.4 实验仪器及型号 19 HYPERLINK \l _bookmark21 2.5 介质阻挡微等离子体物理参数测量 20 HYPERLINK \l _bookmark22 2.5.1 输入电压与输入电流的测量 20 HYPERLINK \l _bookmark23 2.5.2 放电电压、频率及放电电流的测量 20 HYPERLINK \l _bookmark24 2.6 实验结果计算与分析 20 HYPERLINK \l _bookmark25 2.6.1 色谱分析法 20 HYPERLINK