超重力反应器中甘氨酸钠吸收混合气体中CO2的-高校化学工程学报.PDF

第 29 卷第 2 期 高 校 化 学 工 程 学 报 No.2 Vol.29 2015 年 4 月 Journal of Chemical Engineering of Chinese Universities Apr. 2015 文章编号：1003-9015(2015)02-0438-05 超重力反应器中甘氨酸钠吸收混合气体中 CO2 的实验研究 赵晨希, 邹海魁, 初广文, 向 阳 (北京化工大学 教育部超重力工程研究中心, 北京 100029) 摘 要：CO2 减排已经成为国际关注的热点问题。近年来，化学吸收法以其效率高、适应范围广、技术成熟等优点， 逐渐占据主导地位。采用甘氨酸钠溶液为吸收剂，在超重力反应器中进行了 CO2 吸收实验，考察了转速、吸收液温度、 吸收液浓度、气液比等对 CO2 吸收率的影响。结果表明：CO2 的吸收率随着转速的增加而上升，当转速达到 1000 rmin1 后，吸收率基本趋于稳定；CO2 的吸收率随着吸收液温度的升高而升高，在 90 ℃时可以达到 83% 以上；在实验范围内， CO2 的吸收率随吸收液浓度的增加略有增加，随气液比的增加而逐渐降低并趋于稳定。 关键词：二氧化碳；甘氨酸钠；超重力反应器；吸收 中图分类号：TQ028.14 文献标识码：A DOI:10.3969/j.issn.1003-9015.2015.02.030 Study of Carbon Dioxide Absorption by Aqueous Sodium Glycine in a Rotating Packed Bed ZHAO Chen-xi, ZOU Hai-kui, CHU Guang-wen, XIANG Yang (Research Center of the Ministry of Education for High Gravity Engineering and Technology, Beijing University of Chemical Technology, Beijing 100029, China) Abstract: Carbon dioxide emission reduction has become a hot issue and attracted international attention. In recent years, chemical absorption methods gradually dominate the market since they have advantages of high efficiency, widely adaptation and mature technologies. CO2 absorption experiments were conducted in a rotating packed bed using aqueous sodium glycine as a solvent. Effects of rotational speed, concentration and temperature of absorption solution, and gas-liquid ratio on CO2 absorption efficiency were investigated. The experimental results indicate that the absorption efficiency of CO2 increases with the increasing of rotational spe