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Letter
pubs.acs.org/NanoLett
High-Density Carbon Nanotube Buckypapers with Superior
Transport and Mechanical Properties
Ling Zhang, Guang Zhang, Changhong Liu,* and Shoushan Fan
Tsinghua-Foxconn Nanotechnology Research Center and Department of Physics, Tsinghua University, Beijing 100084, People’s
Republic of China
ABSTRACT: High-density buckypapers were obtained by
using well-aligned carbon nanotube arrays. The density of the
buckypapers was as high as 1.39 g cm−3, which is close to the
ultimate density of ideal buckypapers. Then we measured the
transport and mechanical properties of the buckypapers. Our
results demonstrated that its electrical and thermal con-
ductivities could be almost linearly improved by increasing its
density. In particular, its superior thermal conductivity is nearly
twice that of common metals, which enables it a lightweight and more efficient heat-transfer materials. The Young’s modulus of
the buckypapers could reach a magnitude over 2 GPa, which is greatly improved compared with previous reported results. In
view of this, our work provided a simple and convenient method to prepare high-density buckypapers with excellent transport
and mechanical properties.
KEYWORDS: Carbon nanotubes, buckypapers, CNT-based macroscopic materials, thermal conductivity
A ligned carbon nanotube paper, also called aligned on the properties of the aligned buckypaper. Several effective
buckypaper, made from carbon nanotubes (CNTs), methods, such as CNT suspension in strong magnetic fields,
because of its potential
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