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《localized surface plasmon resonanse spectroscopy of single silver nanocubes》.pdf
NANO
LETTERS
Localized Surface Plasmon Resonance 2005
Vol. 5, No. 10
Spectroscopy of Single Silver
Nanocubes
Leif J. Sherry, Shih-Hui Chang, George C. Schatz,* and Richard P. Van Duyne*
Chemistry Department, Northwestern Uniersity, 2145 Sheridan Road,
E anston, Illinois 60208-3113
Benjamin J. Wiley and Younan Xia
Department of Chemistry, Uni ersity of Washington, Seattle, Washington 98195
Received August 10, 2005
ABSTRACT
In this work, we use dark-field microscopy to observe a new plasmon resonance effect for a single silver nanocube in which the plasmon line
shape has two distinct peaks when the particles are located on a glass substrate. The dependence of the resonance on nanocube size and
shape is characterized, and it is found that the bluer peak has a higher figure of merit for chemical sensing applications than that for other
particle shapes that have been studied previously. Comparison of the measured results with finite difference time domain (FDTD) electrodynamics
calculations enables us to confirm the accuracy of our spectral assignments.
The optical properties of metal nanoparticles have been the only to dipolar excitations but also to higher-order multipolar
subject of intensive research efforts because of their applica- excitations for certain nanoparticle structures.16
tions in research areas such a
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