Real-Time Particle Mass Spectrometry Based on Resonant Micro Strings 英文参考文献.docVIP

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Real-Time Particle Mass Spectrometry Based on Resonant Micro Strings 英文参考文献.doc

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Real-Time Particle Mass Spectrometry Based on Resonant Micro Strings 英文参考文献

Sensors2010,10,8092-8100;doi:10.3390/s100908092 OPENACCESS sensors ISSN1424-8220 /journal/sensors Communication Real-TimeParticleMassSpectrometryBasedonResonant MicroStrings SilvanSchmid ,S?renDohnandAnjaBoisen ? DepartmentofMicro-andNanotechnology,TechnicalUniversityofDenmark,DTUNanotech, Building345East,DK-2800KongensLyngby,Denmark;E-Mails:soren.dohn@nanotech.dtu.dk (S.D.);anja.boisen@nanotech.dtu.dk(A.B.) ? Authortowhomcorrespondenceshouldbeaddressed;E-Mail:silvan.schmid@nanotech.dtu.dk; Tel:+45-452-557-32,Fax:+45-458-877-62. Received:10July2010;inrevisedform:30July2010/Accepted:15August2010/ Published:27August2010 Abstract: Micro-andnanomechanicalresonatorsarewidelybeingusedasmasssensors duetotheirunprecedentedmasssensitivity. Wepresentasimpleclosed-formexpression which allows a fast and quantitative calculation of the position and mass of individual particles placed on a micro or nano string by measuring the resonant frequency shifts of the?rsttwobendingmodes.Themethodhasbeentestedbydetectingthemassspectrumof microparticlesplacedonamicrostring. Thismethodenablesreal-timemassspectrometry necessary for applications such as personal monitoring devices for the assessment of the exposuredoseofairbornenanoparticles. Keywords: mass spectrometry; MEMS; NEMS; nanoparticles; string resonator; micro beads;aerosol;particlesensor 1. Introduction In1995theuseofresonantmicrometerscaledcantileversasmasssensorswasproposed[1,2].Since then, cantilever based mass sensors have been shown to have the sensitivity to measure the mass of singlecellsandlargemolecules[3–5]. Theexceptionalmasssensitivityofmicroandnanomechanical resonatorsmakestheminterestingforapplicationssuchasforthedetectionofairbornenanoparticles. The use of nanoparticles in commercial applications has increased and personal monitoring devices Sensors2010,10 8093 for the assessment of nanoparticle exposure doses are demanded due to the still unknown toxic effects[6].Recently,nanobeambasedsensorshavebeenuse