原创力文档锂空电池技术文档Elucidating the Mechanism of Oxygen Reduction for Lithium-Air Battery Applications.pdfVIP
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J.Phys.Chem.C2009,113,20127–2013420127
ElucidatingtheMechanismofOxygenReductionforLithium-AirBatteryApplications
CormacO.Laoire,SanjeevMukerjee,andK.M.Abraham*
DepartmentofChemistryandChemicalBiology,NortheasternUniVersity,360HuntingtonAVenue,
Boston,Massachusetts02115
EdwardJ.PlichtaandMaryA.Hendrickson
U.S.ArmyCERDEC,ArmyPowerDiVision,Ft.Monmouth,NewJersey07703
ReceiVed:August21,2009;ReVisedManuscriptReceiVed:September28,2009
Unlockingthetrueenergycapabilitiesofthelithiummetalnegativeelectrodeinalithiumbatteryhasuntilnow
beenlimitedbythelowcapacityintercalationandconversionreactionsatthepositiveelectrodes.Abrahametal.
(Abraham,K.M.;Jiang,Z.J.Electrochem.Soc.1996,143,1-5)overcamethislimitationbyremovingthese
electrodesandallowinglithiumtoreactdirectlywithoxygenintheatmosphere,formingtheLi-airbattery.The
Li/O2batteryredoxcouplehasatheoreticalspecificenergyof5200Wh/kgandrepresentstheultimate,
environmentallyfriendlyelectrochemicalpowersource.Inthiswork,wereportforthefirsttimetheintimaterole
ofelectrolyte,inparticulartheroleofionconductingsalts,indeterminingthereversibilityandkineticsofoxygen
reductioninnonaqueouselectrolytesdesignedforsuchapplications.Suchfundamentalunderstandingofthishigh
energydensitybatteryiscrucialtoharnessingitsfullenergypotential.ThekineticsandmechanismsofO2reduction
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