《Angular-based spatially resolved laser-induced breakdown spectroscopy： a new technique for the effective enhancement of signals without an external time delay system》.pdfVIP

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《Angular-based spatially resolved laser-induced breakdown spectroscopy： a new technique for the effective enhancement of signals without an external time delay system》.pdf

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《Angular-based spatially resolved laser-induced breakdown spectroscopy： a new technique for the effective enhancement of signals without an external time delay system》.pdf

Chin．Sci．Bul1．(2014)59(27)：3377—3384 csb．scichina．com DOI10．1007／sl1434—014—0399一Y www ．springer．com ／scp Angular-basedspatiallyresolvedlaser-inducedbreakdown spectroscopy：anew techniquefortheeffectiveenhancement ofsignalswithoutanexternaltimedelaysystem QingyuLin。XuWang ‘GuanghuiNiu ‘ HongjanLai·XiaoqinZhu。KunpingLiu ‘ TaoXu 。YixiangDuan Received：12February2014／Accepted：27March2014／Publishedonline：27May2014 @ ScienceChinaPressandSpringer—VerlagBerlinHeidelberg2014 Abstract In thisstudy，wedeveloped anovelangular— Keywords Laser-inducedbrekadownspectroscopy based spatially resolved laser．．induced breakdown spec．． Signalenhancement·Spatialdistribution troscopyrABSR—LIBS)technique．Thisnewmethodallows the spatially resolved spectroscopic propertiesoflaser— inducedplasmatobe investigatedusingdifferentangles 1 Introduction andpolardistanceswithaspatiallya ustablefiberoptics probe．The experimentalevaluationssuggested thatthe Laser—induced breakdown spectroscopy (LIBS) isan intensityoftheAlsigna1distributionsinthe “side—view” increasinglypopulratoolforanalyticalchemistry 【1】．LIBS dependedgreatlyontheangleofthecollectionprobe．The haspotentia1applicationsin qualitativeanalysisand the locationofacollectionprobeat50。wouldfacilitateeffi— semi—quantitativedetemr inationoftheelementalcomposi— cientspectralcollectionandminimizethedisturbanceof tionsofvarioussamples[2—4】，eveninhostileenvironments the plasma plume．The spectralsignalsin the plasma [5—9]．Inthistechnique，abrightplasmaisproducedbythe emissionshad differentdistribution atvraiouspolardis— interactionbetweenalaserpulseandthesamplemateria1． tancesusing the samecollection angle，and the highest Thespectrallinesemittedbytheplasmaarethencollected， signalintensitywasobservedbetween l5and35mm polra