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Behavior ofdissolvedinorganicarsenicintheYellowSeaandEastChinaSea.pdf

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Behavior ofdissolvedinorganicarsenicintheYellowSeaandEastChinaSea

ARTICLE IN PRESS Deep-Sea Research II 57 (2010) 1035–1046Contents lists available at ScienceDirectDeep-Sea Research II0967-06 doi:10.1 n Corr E-mjournal homepage: /locate/dsr2Behavior of dissolved inorganic arsenic in the Yellow Sea and East China SeaJ.L. Ren a,n, J. Zhang b, D.D. Li a, Y. Cheng a, S.M. Liu a a Key Laboratory of Marine Chemistry Theory and Technology, Ministry of Education, Ocean University of China, 238 Songling Road, Qingdao 266100, People’s Republic of China b State Key Laboratory of Estuarine and Coastal Research, East China Normal University, 3663 Zhongshan Road North, Shanghai 200062, People’s Republic of Chinaa r t i c l e i n f o Article history: Received 17 February 2010 Accepted 17 February 2010 Available online 25 February 2010 Keywords: Dissolved arsenic Speciation Yellow Sea East China Sea Distribution45/$ - see front matter 2010 Elsevier Ltd. A 016/j.dsr2.2010.02.005 esponding author. Tel.: +86 532 f ail address: renjingl@ (J.L. Rena b s t r a c t The Yellow Sea and East China Sea are strongly affected by input from freshwater discharge (e.g., from the Changjiang (Yangtze River) in the west and the Kuroshio incursion in the east. The R/V Dong Fang Hong 2 carried out two cruises in September of 2002 and 2003 to understand the behavior of arsenic in the Yellow Sea and East China Sea. Arsenic species (total dissolved inorganic arsenic and arsenite) were determined by selective hydride generation–atomic fluorescence spectrometry. High concentrations of total dissolved inorganic arsenic species (TDIAs; [As(V)]+[As(III)]) appeared near the Changjiang Estuary and at the bottom of the shelf-break in the East China Sea where the incursion of the Kuroshio reaches the shelf. TDIAs were moderately depleted in the surface water and enriched in the deep water. The distribution of arsenite (AsO3 3 , As(III)) was opposite that of arsenate (AsO4 3 , As(V)) in seawater, but was positively correlated with that of Chlorophyll-a. The As(III)/T