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钠离子电池电解液文献.pdf
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Energy C
Environmental Science
Cite this: Energy Environ. Sci., 2012, 5, 8572
/ees PAPER
In search of an optimized electrolyte for Na-ion batteries
Alexandre Ponrouch, *ac Elena Marchante,ac Matthieu Courty,bc Jean-Marie Tarasconbc
*ac
and M. Rosa Palacın
Received 17th May 2012, Accepted 12th June 2012
DOI: 10.1039/c2ee22258b
2 B
1 8
0 5
2 2
r 2 Electrolytes are essential for the proper functioning of any battery technology and the emerging Na-ion
e 2
b E technology is no exception. Hence, a major focus on battery research is to identify the most appropriate
m E
e 2
t C formulation so as to minimize interface reactions and enhance both cell performances and safety
p
e /
9
S 3 aspects. In order to identify suitable electrolyte formulations for Na-ion chemistry we benchmarked
7 0
0 1
.
n 0 various electrolytes containing diverse solvent mixtures (cyclic, acyclic carbonates, glymes) and Na-
o 1
:
S i
o based salts having either F-based or perchlorate anions and measured viscosity, ionic conductivity, and
A d
|
C
, g thermal and electrochemical stability. The binary EC:PC solvent mixture has emerged as the best
s r
c o
i c. solvent formulation and has been used to test the performance of Na/hard carbon cells with b
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