原创力文档conformational effects in non-stoichiometric complexes of two hyperbranched molecules with a linear polyelectrolytenon-stoichiometric复合体的构象影响两个超支化分子与一个线性聚电解质.pdfVIP
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conformational effects in non-stoichiometric complexes of two hyperbranched molecules with a linear polyelectrolytenon-stoichiometric复合体的构象影响两个超支化分子与一个线性聚电解质
Polymers 2012, 4, 240-255; doi:10.3390/polym4010240
OPEN ACCESS
polymers
ISSN 2073-4360
/journal/polymers
Article
Conformational Effects in Non-Stoichiometric Complexes of
Two Hyperbranched Molecules with a Linear Polyelectrolyte
George Dalakoglou 1, Kostas Karatasos 1,*, Sergey Lyulin 2, Sergey Larin 2, Anatoly Darinskii 2
3
and Alexey Lyulin
1 Physical Chemistry Laboratory, Chemical Engineering Department, Aristotle University of
Thessaloniki, 54124 Thessaloniki, Greece; E-Mail: gdalakog@cheng.auth.gr
2 Institute of Macromolecular Compounds, Russian Academy of Sciences, Bolshoi Pr. 31,
199004 St. Petersburg, Russia; E-Mails: s.v.lyulin@ (S.L.); selarin@macro.ru (S.L.);
a.darinskii@mail.ru (A.D.)
3 Theory of Polymers and Soft Matter, Department of Applied Physics, Technische Universiteit
Eindhoven, P.O. Box 513 5600 MB Eindhoven, The Netherlands; E-Mail: a.v.lyulin@tue.nl
* Author to whom correspondence should be addressed; E-Mail: karatas@eng.auth.gr;
Tel.: +30-2310-995-850; Fax: +30-2310-996-222.
Received: 9 December 2011; in revised form: 22 December 2011 / Accepted: 14 January 2012 /
Published: 17 January 2012
Abstract: We report results from Brownian dynamics computer simulations of systems
comprised by two terminally charged hyperbranched molecules preferentially branched
in the periphery, with an oppositely charged linear chain of varying length. Comparison
of the findings from the present study to stoichiometric counterp
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