原创力文档primary no2 emissions and their impact on air quality in traffic environments in germany主要二氧化氮排放及其对德国交通环境空气质量的影响.pdfVIP
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primary no2 emissions and their impact on air quality in traffic environments in germany主要二氧化氮排放及其对德国交通环境空气质量的影响
Kurtenbach et al. Environmental Sciences Europe 2012, 24:21
/content/24/1/21
RESEARCH Open Access
Primary NO2 emissions and their impact on air
quality in traffic environments in Germany
*
Ralf Kurtenbach, Jörg Kleffmann, Anita Niedojadlo and Peter Wiesen
Abstract
Background: The decreasing NOX concentrations at urban measurement stations in Germany are in agreement
with the reduction of NOX emissions from vehicular traffic. However, the measured NO2 concentrations are
stagnating nationwide. In 2010, at more than the half of the urban measurement stations in Germany, annual mean
values for NO exceeded the new Europe-wide limit value of 40 μg/m3 (20 ppbv) NO . Similar findings are reported
2 2
from many other member states of the European Union.
Results: The observed trend of the airborne NO concentrations has different reasons. Firstly, the NO /NO
2 2 x
emission ratio has increased significantly during the last two decades. Furthermore, secondary NO , caused by the
2
titration reactions of NO with ozone (O ) and peroxy radicals (RO ), is responsible for the major fraction
3 2
(approximately 70%) of the measured NO2. However, secondary NO2 shows a highly nonlinear dependency on NOx
and thus, is decreasing much more slowly than expected from the decreasing NOx levels. Based on the results
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