Chapter 9 Photoluminescence Spectroscopy As A Probe For Disorder And Excitonic Effects In Organic And Inorganic Semiconductor英文电子资料.pdf
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CHAPTER 9:
PHOTOLUMINESCENCE SPECTROSCOPY AS A
PROBE FOR DISORDER AND EXCITONIC
EFFECTS IN ORGANIC AND INORGANIC
SEMICONDUCTORS
U. Lemmer a and E. O. Göbel b
aSektion Physik, Ludwig–Maximilians– Universität München, Amalienstr. 54, 80799
München, Germany .
bPhysikalisch–Technische Bundesanstalt, Bundesallee 100,
38023 Braunschweig, Germany .
1. Introduction
2. Method
3. Luminescence dynamics in inorganic model systems
3.1 Bimolecular carrier recombination in a crystalline semiconductor
3.2 Photoluminescence in a strongly disordered semiconductor : Hydrogenated
amorphous silicon
3.3 Excitons localized by disorder
4. Recombination and Relaxation of Photoexcitations in Poly(phenylene vinylene)s
4.1 Recombination dynamics
4.2 Femtosecond energy relaxation
4.3 Monte–Carlo simulations of the photoexcitation dynamics
4.4 The influence of an electric field on the photoluminescence
5. Conclusions and outlook
2 12
1 INTRODUCTION
Time–resolved photoluminescence (PL) spectroscopy has emerged as an important
tool for studying the optical and electronic properties of solid state materials suited for
optoelectronic applications. PL-experiments provide relatively direct information about
recombination and relaxation processes. In general, these experiments are useful for the
investigation of the electronic properties of the excited state and offer several advantages
over other optical techniques. In the context discussed here, the high sensitivity of PL–
spectroscopy and the relative ease to obtain temporal information is of large importance.
The high sensitivity allows to study the PL–behavior over large variations in the excitation
intensity and therefore is a means to explore the low excitation limit as well as nonlinear
effects. The time–resol
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