BTF系统处理硫化氢废气工程设计外文参考文献译文及原文.doc

本科毕业设计(论文) 学 院： 环境科学与工程学院 专 业： 环境工程 年级班别： 200级班 学 号： 310008168 学生姓名： 指导教师： 2008 年 6 月 11 日 Biological sweetening of energy gases mimics in biotrickling filters Marc Fortuny a,c , Juan A. Baeza a, Xavier Gamisans b, Carles Casas a, Javier Lafuente a, Marc A. Deshusses c,*, David Gabriel a,1 a Department of Chemical Engineering, Universitat Auto`noma de Barcelona, Edifici Q, Campus de Bellaterra, 08193 Bellaterra, Barcelona, Spain b Department of Mining Engineering and Natural Resources, Universitat Polite`cnica de Catalunya, Manresa, Spain c Department of Chemical and Environmental Engineering, University of California, Riverside, CA 92520, United States Received 25 July 2007; received in revised form 27 October 2007; accepted 29 October 2007 Available online 21 December 2007 Abstract Removal of hydrogen sulfide from waste and energy-rich gases is required, not only because of environmental health and safety reasons, but also because of operational reasons if such gases have to be used for energy generation. A biotrickling filter for the removal of ultra-high concentrations of H2S from oxygen-poor gases is proposed and studied in this work. Two laboratory-scale biotrickling filters were used to study the startup period and to determine the long-term performance of the gas sweetening process. The inlet H2S concentration ranged from 900 to 12000 ppmv and two different packing materials were investigated. There was no toxicity effect observed even at a the highest H2S concentration, and maximum elimination capacities of 280 and 250 g H2S m-3 h-1 were obtained at gas contact times of 167 and 180 s, respectively. Elemental sulfur and sulfate were found to be the most abundant end-products of the biological oxidation of sulfide when operated under microaerophilic conditions. The biotrickling filter was able to quickly recover its nominal performance after different load increases and system shutdowns s