Field Enhancement - Home Quantum Electronics Group Jack 场增强-家居量子电子集团，杰克.pptVIP

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Field Enhancement - Home Quantum Electronics Group Jack 场增强-家居量子电子集团，杰克.ppt

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Field Enhancement - Home Quantum Electronics Group Jack 场增强-家居量子电子集团，杰克

Near-field Optical Imaging of Carbon Nanotubes Achim Hartschuh, Huihong Qian Tobias Gokus, Department Chemie und Biochemie and CeNS, Universit?t München Neil Anderson, Lukas Novotny The Institute of Optics, University of Rochester, Rochester, NY Why High Spatial Resolution Near-field Optics? Why Near-field Optics? Why Near-field Optics? Why Near-field Optics? ? Diffraction Limit Tip-Enhanced Spectroscopy Tip-Enhanced Spectroscopy Tip-Enhanced Spectroscopy Experimental Setup Confocal microscope Tip-enhanced Spectroscopy Single-Walled Carbon Nanotubes (SWCNT) Graphene sheet + roll up Near-field Raman Imaging of SWCNTs Near-field Raman Spectroscopy Resolution enhancement Signal Enhancement Signal Enhancement Distance Dependence Near-field Raman Spectroscopy Simultaneous Raman and PL Spectroscopy Near-field optical imaging of SWCNTs Localized PL-Emisssion on Glass Near-field PL-Spectroscopy Spatial resolution 15 nm? Signal amplification? Tip as nanoscale ?light source“ Signal Enhancement Signal Enhancement Signal Enhancement (First data) Signal Enhancement (First data) Signal Enhancement Near-field Interactions Uncertainty relation: Diffraction limit for propagating waves: Summary High-resolution optical microscopy of carbon nanotubes using a sharp laser-illuminated metal tip PL and Raman spectroscoy and imaging Spatial resolution 15 nm Signal enhancement Results Resolved RBM variations (IMJ) on the nanoscale Non-uniform emission energies that result from local variations of dielectric environment Strongly confined emission signals ? bound excitons? PL-Quantum yield can be enhanced by metal tip Thanks to Acknowledgement PC Tuebingen: Alfred J. Meixner Mathias Steiner Antonio Virgilio Failla Funding: DFG, Cm Siegen, NSF, FCI PC Siegen: Gregor Schulte PC Tuebingen: Alfred J. Meixner Mathias Steiner Antonio Virgilio Failla Funding: DFG, Cm Siegen, NSF, FCI PC Siegen: Gregor Schulte cnt are very particular material, at least for spectros