某铀矿区水稻土—地表水铀含量对稻米铀含量的影响向龙1a1b.DOC

某铀矿区水稻土地表水铀含量对稻米铀含量的影响 向龙1a,1b，刘平辉1a,1b，张淑梅2，魏长帅3 (1.东华理工大学，a 地球科学学院，b，南昌 33001； 2.江西有色地质勘查二队，江西 赣州 34100；3.安徽省地质矿产勘查局326地质队，安徽 安庆 246000) 摘要：以水稻土—地表水铀含量为视角，从水稻土剖面铀含量分布规律、水稻土与下伏岩体稀土元素特征、不同河流不同河段水稻土—地表水—稻米铀含量特征、水稻土与稻米铀含量关系4个方面研究721铀矿区稻米铀含量成因。结果表明，水稻土剖面铀含量从表层至半风化花岗质基岩层呈明显降低的特征，说明水稻土铀含量高的原因不是土壤母质铀含量高；岩石与水稻土稀土元素标准化模式均表现为向右倾斜型，均属轻稀土富集型，轻稀土分馏明显，表明水稻土为还原环境，吸附作用较强；不同河流不同河段水稻土—地表水—稻米铀含量平均值的特性均为上游最低、中游最高、下游次之。铀矿区地表水环境符合铀元素在水稻土中被平衡吸附的动力学条件，有利于铀元素在矿区内河流中游地区的水稻土中沉淀富集；正在采矿区水稻土与稻米铀含量具有高度的空间耦合性，呈指数正相关关系，相关系数0.749。矿区内河流沿岸稻米铀含量的分布特征是由铀元素的迁移途径决定的“采矿活动（铀尾矿露天堆放）→地表水→水稻土”。 关键词：铀矿区；稻米；铀含量；水稻土；地表水；成因；铀迁移 文献标志码：A 文章编号：1007-7545（2018）07-0000-00 Effect of Uranium Contents of Paddy Soil and Surface Water on Uranium Contents of Rice in a Uranium Mining Area XIANG Long1a,1b, LIU Ping-hui1a,1b, ZHANG Shu-mei2, WEI Chang-shuai3 (a. College of Earth Sciences, b. State Key Laboratory Breeding Base of Nuclear Resources and Environment, Ministry of Education, 1. East China University of Technology, Nanchang 330013, China； 2. No.2 Team of Jiangxi Nonferrous Metal Geological Exploration Bureau, Ganzhou 341000, Jiangxi, China； 3. Geological Team 326 of Geology and Mineral Exploration Bureau in Anhui Province, Anqing 246000, Anhui, China) AbstractIn order to explore contributing factors for uranium contents in rice of a uranium mining area, distribution of uranium contents in paddy soil profiles, REE characteristics in paddy soils and underlying bedrock, characteristics of uranium contents of paddy soil, surface water, and rice in different reaches of two rivers, and relationship between uranium contents of paddy soils and rice were investigated from perspective of uranium content characteristics in paddy soil and surface water. The results show that uranium contents of paddy soil profiles significantly drop from surface of paddy soil to semi-weathering of granitic bedrock, which means high uranium content in paddy soil is not due to high content of uranium in the soil parent material. The normalized p