2019年某铀尾矿中U、Th在电场作用下释放及迁移规律.docVIP

doi：10.3969/j.issn.1007-7545.2019.02.015某铀尾矿中U doi：10.3969/j.issn.1007-7545.2019.02.015 李稳，陈功新，孙占学，刘顺亮，王文凤 （东华理工大学 水资源与环境工程学院，南昌 330013） 摘要：以电流场作为核素迁移的载体，研究某铀尾矿中U、Th在0、0.5、1.0、1.5 V/cm直流电场条件下的释放及迁移规律。结果表明，在添加电场时，铀元素的浸出量小于自然淋滤条件下的浸出量，但土壤对铀的释放能力明显提升，且电场强度越强，释放能力越强，而钍元素则受其影响不大。在0、0.5、1.0、1.5 V/cm电场强度条件下铀元素的累积浸出量分别为1.439、1.285、1.474、1.795 mg/L，说明电场强度对U的释放以及迁移有促进作用。铀元素在电场作用下的迁移规律和其他重金属元素的规律类似，都是阳极往阴极迁移，且电场强度越大，阳极附近富集的铀元素浓度越高。矚慫润厲钐瘗睞枥庑赖賃軔朧碍鳝绢懣硯涛镕頃赎巯驂雞虯从躜鞯烧。 关键词：核素迁移；铀尾矿；电动修复；放射性核素 中图分类号：X758 文献标志码：A 文章编号：1007-7545（2019）02-0000-00聞創沟燴鐺險爱氇谴净祸測樅锯鳗鲮詣鋃陉蛮苎覺藍驳驂签拋敘睑绑。 Release and Migration of U and Th in Uranium Tailings under Electric Field残骛楼諍锩瀨濟溆塹籟婭骒東戇鳖納们怿碩洒強缦骟飴顢歡窃緞駔蚂。 LI Wen, CHEN Gong-xin, SUN Zhan-xue, LIU Shun-liang, WANG Wen-feng酽锕极額閉镇桧猪訣锥顧荭钯詢鳕驄粪讳鱸况閫硯浈颡閿审詔頃緯贾。 (School of Water Resources and Environmental Engineering, East China University of Technology, Nanchang 330013, China)彈贸摄尔霁毙攬砖卤庑诒尔肤亿鳔简闷鼋缔鋃耧泞蹤頓鍥義锥柽鳗铟。 Abstract：With current field as carrier of nuclide migration, release and migration of U and Th in uranium tailings under different DC electric fields of 0, 0.5, 1.0 and 1.5 V/cm were investigated. The results show that leaching amount of uranium in electric field is lower than that of natural leaching conditions, but uranium release ability from soil under electric field is significantly improved, and the stronger the electric field intensity, the stronger the release ability is, while Th element is not affected. Cumulative leaching amount of uranium element is 1.439, 1.285, 1.474, and 1.795 mg/L respectively under electric field of 0, 0.5, 1.0 and 1.5 V/cm, which indicates that electric field promotes release and migration of U. Uranium element moves from anode toward cathode under electric field, which is similar to that of other heavy metal elements. The higher the electric field intensity, the higher the concentration of uranium enriched near the anode is.謀荞抟箧飆鐸怼类蒋薔點鉍杂篓鳐驱數硯侖葒屜懣勻雏鉚預齒贡缢颔。 Key words：nuclides migration; uranium tailings; electric repair; radionuclid