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Synthesis_2016_Hua_Fu_review_-_Copper-Catalyzed_Coupling_Reactions.pdf
ACCOUNT 745
Copper-Catalyzed Coupling Reactions
Copper-Catalyzed Coupling ReactionsHonghua Rao, Hua Fu*
Key Laboratory of Bioorganic Phosphorus Chemistry and Chemical Biology (Ministry of Education), Department of Chemistry,
Tsinghua University, Beijing 100084, P. R. of China
Fax +86(10 E-mail: fuhua@mail.tsinghua.edu.cn
Received 11 November 2010
1 Introduction and Background
Abstract: This account summarizes our recent developments in
copper-catalyzed coupling reactions, including copper-catalyzed N-,
O-, and P-arylations, the formation of carbon–nitrogen and carbon– Transition-metal-catalyzed cross-coupling reactions are
carbon bonds via carbon–hydrogen bond activation, and the synthe- universal protocols in organic synthesis, and they provide
sis of N-heterocyclic compounds. highly efficient transformations and allow the straightfor-
ward, high-yielding, and scalable syntheses of organic
1 Introduction and Background compounds. In particular, the tolerant reactions can intro-
2 Copper-Catalyzed N-, O-, and P-Arylations duce certain functional groups with surgical precision.1
2.1 Copper-Catalyzed Synthesis of Primary Aromatic Amines
2.2 Copper-Catalyzed Synthesis of Phenols in Water Among such transition-metal-catalyzed cross-couplings,
2.3 Copper-Catalyzed N-Arylation of Aliphatic Amines and copper plays a significant role, and its use has greatly in-
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