Light scattering properties of sea-salt aerosol particles inferred from modeling studies and ground.pdf
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Light scattering properties of sea-salt aerosol particles inferred from modeling studies and ground
ARTICLE IN PRESSJournal of Quantitative Spectroscopy 0022-4073/$ - se
doi:10.1016/j.jq
Correspond
E-mail addrRadiative Transfer 101 (2006) 498–511
/locate/jqsrtLight scattering properties of sea-salt aerosol particles inferred
from modeling studies and ground-based measurements
K. Chamaillard, C. Kleefeld, S.G. Jennings, D. Ceburnis, C.D. O’Dowd
Atmospheric Research Group, Department of Physics, National University of Ireland, Galway, IrelandAbstract
Direct climate radiative forcing depends on the aerosol optical depth t, the single scattering albedo $, and the up-scatter
fraction b; these quantities are functions of the refractive index of the particles, their size relative to the incident
wavelength, and their shape. Sea-salt aerosols crystallize into cubic shapes or in agglomerates of cubic particles under low
relative humidity conditions. The present study investigates the effects of the shape of dried sea-salt particles on the
detection of light scattering from the particles. Ground-based measurements of scattering and backscattering coefficients
have been performed with an integrating nephelometer instrument for a wavelength l ? 0:55mm. The measurements are
compared to two models: the Mie theory assuming a spherical shape for the particles and the Discrete Dipole
Approximation (DDA) model for the hypothesis of cubic shape of the sea-salt aerosols. The comparison is made
accurately by taking into account the actual range of the scattering angles measured by the nephelometer in both models
that is from 71 to 1701 for the scattering coefficient and from 901 to 1701 for the backscattering coefficient. Modeled
scattering and backscattering coefficients increase for nonspherical particles compared to spherical shape of particles with
diameter larger than about 1 mm. However, the comparison of the modeling results with the measurements gives best
agreement for particles diameter less than about 1mm. The size distribution of the particles is measured with two
instru
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