NH4+交换度对 CuY催化剂上甲醇氧化羰基化反应性能的影响.pdfVIP

Chinese Journal of Catalysis 37 (2016) 1403–1412 催化学报 2016年 第37卷 第8期 |   a v a i l a b l e  a t  w w w . s c i e n c e d i r e c t . c o m   j o u r n a l  h o m e p a g e :  w w w . e l s e v i e r . c o m / l o c a t e / c h n j c   Article   Effect of NH4+ exchange on CuY catalyst for oxidative carbonylation of methanol a,b a a, Yuchun Wang , Huayan Zheng , Zhong Li * a Key Laboratory of Coal Science and Technology of Ministry of Education and Shanxi Province, Taiyuan University of Technology, Taiyuan 030024, Shanxi, China b Department of Applied Chemistry, Yuncheng University, Yuncheng 044000, Shanxi, China   A R T I C L E I N F O A B S T R A C T Article history:   NaY and ion exchanged NaNHY zeolite with NH NO were used as the support to prepare CuY cata‐ 4 4 3 Received 4 May 2016 lysts by a high temperature anhydrous interaction between the support and copper (II) acety‐ Accepted 15 June 2016 lacetonate Cu(acac) . The catalysts were used for the oxidative carbonylation of methanol to dime‐