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【Nano2014.3.14】Oriented Assembled TiO 2 Hierarchical Nanowire Arrays with Fast
Letter
/NanoLett
Oriented Assembled TiO2 Hierarchical Nanowire Arrays with Fast
Electron Transport Properties
Xia Sheng,† Dongqing He,† Jie Yang, † Kai Zhu,*,‡ and Xinjian Feng*,†
†Suzhou Institute of Nano-Tech and Nano-Bionics, Chinese Academy of Sciences, Suzhou 215123, Jiangsu, China
‡National Renewable Energy Laboratory, Golden, Colorado 80401, United States
S
*Supporting Information
ABSTRACT: Developing high surface area nanostructured
electrodes with rapid charge transport is essential for artificial
photosynthesis, solar cells, photocatalysis, and energy storage
devices. Substantial research efforts have been recently focused
on building one-dimensional (1D) nanoblocks with fast charge
transport into three-dimensional (3D) hierarchical architec-
tures. However, except for the enlargement in surface area,
there is little experimental evidence of fast electron transport
in these 3D nanostructure-based solar cells. In this
communication, we report single-crystal-like 3D TiO2
branched nanowire arrays consisting of 1D branch epitaxially
grown from the primary trunk. These 3D branched nanoarrays
not only demonstrate 71% enlargement in large surface area (compared with 1D nanowire arrays) but also exhibit fast charge
transport property (comparable to that in 1D single crystal nanoarrays), leading to 52% improvement in solar conversion
efficiency. The orientated 3D assembly strategy reported here can be extended to assemble other metal oxides with one or
multiple components and thus r
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