掺二氧化钛微晶聚集体的若丹明6G溶液的低阈值激射3.pdf

　《激光杂志》1998 年第 19 卷第 1 期 　　　　　　　LASER JOURNAL (Vol 19 ,No 11998) 　　 27 掺二氧化钛微晶聚集体的若丹明 6 G 溶液的低阈值激射 汪河洲 　赵福利 　何拥军 　黄旭光 　　　　　　　　吴明女每 ( ) ( ) 中山大学超快速激光光谱学国家重点实验室 ,广州 　510275 　 中山大学化学系 ,广州 　510275 提要 : 本文实验表明 ,在若丹明 6 G 染料溶液存在二氧化钛微晶团聚体形成的聚集体时 ,染料溶液的激射 阈值比纯净的染料溶液的激射阈值降低20 多倍。激射脉宽接近激发激光脉宽 ,激射谱带很窄并随激发强度 增大而稍微红移和稍微增宽。本文讨论了这种低阈值激射的机制。 关键词 :激射阈值 ,激射光谱 ,瞬态特性 ,分数维 ,微晶聚集体 ,激光染料 Low threshold lasing of rhodamine 6 G solution embeded with TiO2 nanocrystal aggregate W ang Hez hou , Zhao Fuli 　He Yongjun 　Huang X u guang ( State Key Laboratory of Ultrafast Laser Spectroscopy ,Zhongshan University , Guangzhou 　510275) W u Mingmei (Department of Chemistry ,Zhongshan University , Guangzhou 　510275) Abstract : The experimental resuts in this paper show that the lasing threshold of rhodamine 6 G solution ,in which TiO2 nanocrystal aggregate is embeded ,is significantly reduced compared to that of a neat dye solution. The lasing spectral bandwidth of rhodamine 6 G solution embeded with TiO nanocrystal aggregate is very sharp ,and its 2 peak wavelength redshifts slightly according to the increasement of pump density. The emission duration is as short as the pump pulse duration. The mechanism of this low threshold lasing is discussed. Key words :lasing threshold ,lasing spectrum ,transient behavior ,fractal ,nanocrystal aggregate ,laser dye 展波段 ,零维纳米微粒的激射、及其光电子学 1 　引言 和非线性光学特性的研究受到重视。例如 当前 ,激光与光电子学发展的主要方向