原创力文档photoresponsive block copolymers containing azobenzenes and other chromophores光敏嵌段共聚物含有偶氮苯生色团.pdfVIP
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photoresponsive block copolymers containing azobenzenes and other chromophores光敏嵌段共聚物含有偶氮苯生色团
Molecules 2010, 15, 570-603; doi:10.3390/molecule
OPEN ACCESS
molecules
ISSN 1420–3049
/journal/molecules
Review
Photoresponsive Block Copolymers Containing Azobenzenes
and Other Chromophores
Haifeng Yu 1,* and Takaomi Kobayashi 2
1 Top Runner Incubation Center for Academia-Industry Fusion, Nagaoka University of Technology,
1603-1 Kamitomioka, Nagaoka 940-2188, Japan
2 Department of Materials Science and Technology, Nagaoka University of Technology, 1603-1
Kamitomioka, Nagaoka 940-2188, Japan; E-Mail: takaomi@nagaokaut.ac.jp
* Author to whom correspondence should be addressed; E-Mail: yuhaifeng@mst.nagaokaut.ac.jp;
Tel.: +81 0258-47-9310; Fax: +81 0258-47-9300.
Received: 25 December 2009; in revised form: 11 January 2010 / Accepted: 25 January 2010 /
Published: 26 January 2010
Abstract: Photoresponsive block copolymers (PRBCs) containing azobenzenes and other
chromophores can be easily prepared by controlled polymerization. Their photoresponsive
behaviors are generally based on photoisomerization, photocrosslinking, photoalignment
and photoinduced cooperative motions. When the photoactive block forms mesogenic
phases upon microphase separation of PRBCs, supramolecular cooperative motion in
liquid-crystalline PRBCs enables them to self-organize into hierarchical structures with
photoresponsive features. This offers novel opportunities to photocontrol microphase-
separated nanostructures of well-defined PRBCs and extends their diverse applications i
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