proton content and nature in perovskite ceramic membranes for medium temperature fuel cells and electrolysers质子的内容和性质在钙钛矿陶瓷膜介质温度燃料电池和电解槽.pdfVIP

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proton content and nature in perovskite ceramic membranes for medium temperature fuel cells and electrolysers质子的内容和性质在钙钛矿陶瓷膜介质温度燃料电池和电解槽.pdf

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proton content and nature in perovskite ceramic membranes for medium temperature fuel cells and electrolysers质子的内容和性质在钙钛矿陶瓷膜介质温度燃料电池和电解槽

Membranes 2012, 2, 493-509; doi:10.3390/membranes2030493 OPEN ACCESS membranes ISSN 2077-0375 /journal/membranes Article Proton Content and Nature in Perovskite Ceramic Membranes for Medium Temperature Fuel Cells and Electrolysers Philippe Colomban *, Oumaya Zaafrani and Aneta Slodczyk LADIR, UMR7075 CNRS, Université Pierre et Marie Curie (UPMC), 4 Place Jussieu, Paris 75005, France; E-Mails: zaafrani@glvt-cnrs.fr (O.Z.); slodczyk_aneta@ (A.S.) * Author to whom correspondence should be addressed; E-Mail: philippe.colomban@upmc.fr; Tel.: +33-144-272-785; Fax: +33-144-273-021. Received: 28 April 2012; in revised form: 8 June 2012 / Accepted: 28 June 2012 / Published: 25 July 2012 Abstract: Recent interest in environmentally friendly technology has promoted research on green house gas-free devices such as water steam electrolyzers, fuel cells and CO /syngas converters. In such applications, proton conducting perovskite ceramics appear 2 especially promising as electrolyte membranes. Prior to a successful industrial application, it is necessary to determine/understand their complex physical and chemical behavior, especially that related to proton incorporation mechanism, content and nature of bulk protonic species. Based on the results of quasi-elastic neutron scattering (QNS), thermogravimetric analysis (TGA), Raman and IR measurements we will show the complexity of the protonation pro