龚旗煌-飞秒时间分辨测量与应用2.ppt

-- Time related amplification Demonstration of Amplification Ability (荧光放大) Advantages: 半导体量子阱中的载流子扩散 DCM @ 3?10-4mol/l, excitation @ 400nm 系统放大率： 107，将适用于超快生命过程研究 A new technique with ultrafast time resolution and high efficiency Simple in design Wide spectrum range Weak signal amplification Conversion of IR signal to visible range 4、 Femtosecond - SNOM system 100fs time-resolved transmission for GaAs nano-particle ( 100nm) 超短时间和空间小尺度相结合，研究在四维小尺度下的物理新现象和新内容。 Dye Laser 100fs Fiber BBO Chopper UV Filter Variable Delay A B Lock-in PD1 PD2 SNOM Tip Sample 近场双波长超快泵浦—探测 实验系统 探针在硒化镉纳米团簇薄膜表面不同位置得到的泵浦—探测弛豫过程曲线 A,B,C分别为探光延迟泵光0ps,1.2ps和2ps的泵浦—探测图像, D为同时得到的形貌像。 近场双波长超快泵浦—探测 GaAs/AlGaAs量子阱 50keV Ga Ions FIB implantation Patterned t ? 10ps Unpatterned t ? 100ps With ultrafast lasers one can directly observe the carrier spin dynamics in the time domain. Shown above is time-resolved NSOM data from a patterned digital magnetic heterostructure. The microscope scanned across a single line on the sample as the time delay between a pump and a probe pulse was increased from 0-20 picoseconds. Note that one axis is time and the other is distance. The amplitude of the signal is indicative of the number of carriers remaining. The sample was implanted with lines of gallium atoms, which introduce lattice damage. As can be seen, implanted areas have a greatly decreased quantum efficiency and lifetime. ZnSe/Zn0.8Gd0.2Se 6nm Single GaAs QW DRQWR(td)/R0 = [DR(y=0, td)- DR(y=1.5mm, td)]/R0 光产生载流子速度200fs 200fs 纳米量子线研究 300 400 500 600 700 800 900 1000 10 100 1000 Intensity (a. u. ) Wavelength (nm) 800nm、100fs、10mJ的飞秒强激光非聚焦通过水时所产生的超连续光。水中超连续光的产生机制一般有四光子参量过程、自相位调制及受激拉曼效应等。中间的白斑称为白光，由于它具有与入射激光相近的脉冲宽度和极宽的光谱范围，因此可用作泵浦—探测中的探测光，以获得更多样品内部各种动力学过程的信息。 800nm、130fs、2mJ的飞秒强激光经f =6.5cm的透镜聚焦于水中所产生的白光光谱。覆盖了400nm到1000nm的光谱范围，峰值仍位于800nm，在633nm处的白光因部分分解为激光光子和水的拉曼模而出现一个坑（ dip ）。 5、飞秒白光的产生及其光谱应用 * * * * * * * 第四讲、飞秒时间分辨测量II 超快超强激光物理学 任课老师：龚旗煌 (北京大学） 张 杰（物理所） 一、