原创力文档Black carbon and polycyclic aromatic hydrocarbons （PAHs） in surface sediments of China＇s marginal seas.pdf
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Black carbon and polycyclic aromatic hydrocarbons （PAHs） in surface sediments of China＇s marginal seas
ChineseJournalofOceanologyandLimnology
Vo1．27No．2，R 297—308，2009
DOI：1O．1O07／s00343-008-0151．z
Blackcarbonandpolycyclicaromatichydrocarbons(PAHs)
insurfacesedimentsofChina’smarginalseas冰
KANGYanju(康延菊)”，wANGXuchen(王旭晨)卅，，DAIMinhan(戴民汉)””，
FENGHuan(冯桓)卅”，LIAnchun(李安春)，SONGQian(宋茜)
DepartmentofMarineEcolog3’andEnvironmentalStudies，InstituteofOceanologyChineseAcademyofSciences，Qingdao
266071．China
”GraduateSchoolofChineseAcademyofSciences，Beijing100039,China
”DepartmentofEnvironmental，EarthandOceanSciences，UniversiOofMassachusettsatBoston，BostonMA02120，USA
”StateKeyLaboratoryofMarineEnvironmentalScience，XiamenUniversity,Xiamen361005，China
””DepartmentofEarthandEnvironmentalStudies．MontclairStateUniversiyt,MontclairNJ07043．USA
ReceivedJuly9，2008；revisionacceptedOct．21，2008
Abstract Thisstudyinvestigatesthedistributionofblackcarbon(BC、anditscorrelationwithtotal
polycyclicaromatichydrocarbonsf∑PAH、inthesurfacesedimentsofChina’smarginalseas．BC content
rangesfrom 0．10to2．45ITg【／gdw(gramsdryweight)inthesedimentsstudied，andvariedamongthe
differentcoastalregions．TheBohaiBaysedimentshadthehighestBCcontents(average2．18mg／gdw)．
whichcomprisesasignificantfraction(27％—4l％)ofthetotalorganiccrabonfTOC)preservedinthe
sediments．Incomparison，BC inthesurfacesedimentsoftheNorthYellow Sea，JiaozhouBay，EastChina
SeaandtheSouthChinaSeaisleSSabundantandaccountedforanaverageof6％，8％．14％ and5％．
respectively,ofthesedimentaryorganiccarbonpoo1．Theconcentrationof∑PAH inthesurfacesediments
rangesrfom41to3667ng／gdwandshowedlargespatialvariationsamongthesamplingsitesofdifferent
costalregions．TheBohaiBayhasthehighest∑PAH values．rangingfrom 79to3667ng／gdw．This
refleetsthehigh anthropogenicallycontaminated natureofthesedimentsin thebay．BC ispositively
correlatedtoTOCbutastrongcorrelationjsnotfoundbetweenBC and ∑PAH inthesurfacesediments
studied，suggestingthatBC andPAHspreservedinthesedimentsarederivedfrom differentsourcesand
controlledbydifierentbiogeochemicalprocesses．Ours
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