单乙醇胺碳捕集工艺大规模工业化应用提高非平衡级速率模型预测精度.pdf

Engineering 3 (2017) 232–243 Contents lists available at ScienceDirect Engineering journal homepage: /locate/eng Research Smart Process Manufacturing—Article Improving Prediction Accuracy of a Rate-Based Model of an MEA-Based Carbon Capture Process for Large-Scale Commercial Deployment Xiaobo Luo, Meihong Wang* Department of Chemical and Biological Engineering, The University of Sheffield, Sheffield S1 3JD, UK a r t i c l e i n f o a b s t r a c t Article history: Carbon capture and storage (CCS) technology will play a critical role in reducing anthropogenic carbon Received 13 November 2016 dioxide (CO2 ) emission from fossil-fired power plants and other energy-intensive processes. However, the Revised 17 January 2017 increment of energy cost caused by equipping a carbon capture process is the main barrier to its commer- Accepted 30 January 2017 cial deployment. To reduce the capital and operating costs of carbon capture, great efforts have been made Available online 17 March 2017 to achieve optimal design and operation through process modeling, simulation, and optimization. Accurate models form an essential foundation for this purpose. This paper presents a study on developing a more Keywords: accurate rate-based model in Aspen Plus® for the monoethanolamine (MEA)-based carbon capture process Process modeling by multistage model validations. The modeling