Reaction pathways of model compounds of biomass-derived oxygenates on FeNi bimetallic surfaces》.pdf
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Reaction pathways of model compounds of biomass-derived oxygenates on FeNi bimetallic surfaces》.pdf
Surface Science 640 (2015) 159–164
Contents lists available at ScienceDirect
Surface Science
journal homepage: /locate/susc
Reaction pathways of model compounds of biomass-derived oxygenates
on Fe/Ni bimetallic surfaces
Weiting Yu, Jingguang G. Chen ⁎
Department of Chemical Engineering, Columbia University, New York, NY 10027, United States
a r t i c l e i n f o a b s t r a c t
Available online 29 January 2015 Controlling the activity and selectivity of converting biomass-derivatives to fuels and valuable chemicals is critical
for the utilization of biomass feedstocks. There are primarily three classes of non-food competing biomass, cellulose,
Keywords: hemicellulose and lignin. In the current work, glycolaldehyde, furfural and acetaldehyde are studied as model
Bimetallic surfaces compounds of the three classes of biomass-derivatives. Monometallic Ni(111) and monolayer (ML) Fe/Ni(111)
ML Fe/Ni(111) surface bimetallic surfaces are studied for the reaction pathways of the three biomass surrogates. The ML Fe/Ni(111) surface
Biomass-derivatives
is identified as an efficient surface for the conversion of biomass-derivatives from the combined results of density
Furfural
functional theory (DFT) calculations and temperature programmed desorption (TPD) experiments. A correlation
Glycolaldehyde
Acetaldehyde is also es
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