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Selective Oxidation of PM over Li Doped Potassium Titanate Catalysts.pdf
ChinaPetroleum ProcessingandPetrochemicalTechnology
CatalystResearch 2012,Vo1.14,No.2,PP50—54 June30,2012
— —
SelectiveOxidationofPM overLiDopedPotassium
TitanateCatalysts
DuanLinhai
MengXiuhong;GaoYuan;WangQiang;
LiaoningShihuaUniversity,Fushun
(.KeyLaboratoryofPetrochemicalCatalyticScienceandTechnology,
113001. R.China,"2.DepartmentofChemistry,UniversityofOxford,Oxford,OX13TA,UnitedKingdom)
Abstract:K2Ti205andLiK2_ Ti205sampleswithvaryingKcontents 0.125,0.15,0.3),targetedonremovaloftwomain
x
environmentalpollutants:PM andNO weresynthesizedbythesolidstatemethodusingTiO2,KNO3andLiOH H‘2O as
starringmaterialsandwerecharacterizedbyX—raydiffractometry,scanningelectronmicroscopy,andBET.Thecatalytic
activitvoftitanatecatalystsonPM oxidationwasevaluatedusingthetemperatureprogrammedoxidation(TPO)method.
Thetestresuitsshowedthattheperovskitestructureof Ti205wasstillretainedafterdopingasmallamountofLi,andthe
catalyticperformanceofLiK2.Ti205hadbeenimprovedsignificantlycomparedwiththatofK2Ti205.Li015KfssTi205cata—
lysthadthehighestcatalyticactivitywithanignitiontemperatureof210℃ andapeaktemperatureof290℃.Thecatalytic
activityofbothK,Ti,O andLixK2Ti2O5underintimatecontactwashigherthanthatunderloosecontact.W hentheexhaust
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