Degradation of 2,4-Dichlorophenoxyacetic Acid (2,4-D) by Novel Photocatalytic Material of Tourmaline-Coated TiO2 Nanoparticles Kinetic Study and Model.docVIP

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Degradation of 2,4-Dichlorophenoxyacetic Acid (2,4-D) by Novel Photocatalytic Material of Tourmaline-Coated TiO2 Nanoparticles Kinetic Study and Model.doc

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Degradation of 2,4-Dichlorophenoxyacetic Acid (2,4-D) by Novel Photocatalytic Material of Tourmaline-Coated TiO2 Nanoparticles Kinetic Study and Model

Materials 2013, 6, 1530-1542; doi:10.3390/ma6041530 OPEN ACCESS materials ISSN 1996-1944 /journal/materials Article Degradation of 2,4-Dichlorophenoxyacetic Acid (2,4-D) by Novel Photocatalytic Material of Tourmaline-Coated TiO2 Nanoparticles: Kinetic Study and Model 1,2 Xuesen Bian , Jianqiu Chen 1,3,* and Rong Ji 1,* 1 State Key Laboratory of Pollution Control and Resource Reuse, School of the Environment, Nanjing University, Nanjing 210023, China; E-Mail: woshjc@163.com 2 Nanjing Institute of Environmental Sciences of the Ministry of Environmental Protection of PR China, Nanjing 210042, China 3 Department of Environmental Science Department of Analytical Chemistry, China Pharmaceutical University, Nanjing 210009, China * Authors to whom correspondence should be addressed; E-Mails: njcjq@ (J.C.); njudoc@163.com (R.J.); Tel./Fax: +86-131-6007-5092 (R.J.). Received: 19 February 2013; in revised form: 28 March 2013 / Accepted: 7 April 2013 / Published: 15 April 2013 Abstract: The novel complex photocatalytic material was prepared by coating TiO2 nanoparticles on tourmaline using the sol-gel method, and used in the degradation of the herbicide 2,4-D. The results indicated that coating TiO with tourmaline enhanced the 2 photocatalytic activity significantly. Based on the research of a simplified model for the average light intensity in the photoreactor, the influence of the concentration of photocatalyst, and the initial concentration of 2,4-D, a model for the degradation of 2,4-D by the tourmaline-coated TiO nanoparticles was established. Further tests showed that results 2 calculated from this model were close to those obtained in the actual experiments. Keywords: novel photocatalytic material; tourmaline; TiO ; 2,4-D; model 2 1. Introduction Photocatalysis has drawn a lot of attention in environmental application in recent years [1]. Removal of pollution from the environment usin