Controlled Release from Core-Shell Nanoporous Silica Particles for Corrosion Inhibition of Aluminum Alloys英文文献资料.docVIP

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Controlled Release from Core-Shell Nanoporous Silica Particles for Corrosion Inhibition of Aluminum Alloys英文文献资料.doc

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Controlled Release from Core-Shell Nanoporous Silica Particles for Corrosion Inhibition of Aluminum Alloys英文文献资料

HindawiPublishingCorporation JournalofNanomaterials Volume2011,ArticleID760237,10pages doi:10.1155/2011/760237 ResearchArticle ControlledReleasefromCore-ShellNanoporousSilicaParticles forCorrosionInhibitionofAluminumAlloys NanguoLiu, HuifangXu, ShailendraRathod, XingmaoJiang,1,2Ying-BingJiang,3 4 5 1 andC.JeffreyBrinker 1,6 PratikShah, 1 1 DepartmentofChemicalandNuclearEngineeringandCenterforMicro-EngineeredMaterials, UniversityofNewMexico,Albuquerque,NM87106,USA 2 AerosolandRespiratoryDosimetryProgram,LovelaceRespiratoryResearchInstitute,2425RidgecrestDr.SE, Albuquerque,NM87108,USA 3 4 5 6 TransmissionElectronMicroscopyLabs,TheUniversityofNewMexico,Albuquerque,NM87131,USA SCBInnovationAccelerator,DowCorningCorporation,2200W.SalzburgRoad,P.O.Box0994,Midland,MI48686,USA DepartmentofGeoscience,UniversityofWisconsin-Madison,Madison,WI53706,USA AdvancedMaterialLaboratory,SandiaNationalLaboratories,Albuquerque,NM87185,USA CorrespondenceshouldbeaddressedtoC.Je?reyBrinker,cjbrink@ Received3November2010;Accepted2December2010 AcademicEditor:HughD.Smyth Copyright?2011XingmaoJiangetal.ThisisanopenaccessarticledistributedundertheCreativeCommonsAttributionLicense, whichpermitsunrestricteduse,distribution,andreproductioninanymedium,providedtheoriginalworkisproperlycited. Cerium(Ce)corrosioninhibitorswereencapsulatedintohexagonallyorderednanoporoussilicaparticlesviasingle-stepaerosol- assistedself-assembly.Thecore/shellstructuredparticlesaree?ectiveforcorrosioninhibitionofaluminumalloyAA2024-T3. Numerical simulation proved that the core-shell nanostructure delays the release process. The e?ective di?usion coe?cient elucidatedfromreleasedataformonodisperseparticlesinwaterwas1.0×10?14 m sforCe m sforNaCl. 2 3+ 2 comparedto2.5×10?13 Theporesize,poresurfacechemistry,andtheinhibitorsolubilityarecrucialfactorsfortheapplication.Microporoushydrophobic particlesencapsulatingalesssolublecorrosi