原创力文档Calculation of the visible-UV absorption spectra of hydrogen sulfide, bisulfide, polysulfides, and As and Sb sulfides, in aqueous solution.docVIP
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Calculation of the visible-UV absorption spectra of hydrogen sulfide, bisulfide, polysulfides, and As and Sb sulfides, in aqueous solution
Calculationofthevisible-UVabsorptionspectraofhydrogen
sul?de,bisul?de,polysul?des,andAsandSbsul?des,in
aqueoussolution
J.A.Tossell
DepartmentofChemistryandBiochemistry,UniversityofMaryland,CollegePark,
MD20742.E-mail:tossell@
Article
Paper
Received6thMay2003,Accepted28thOctober2003
PublishedasanAdvanceArticleontheweb11thNovember2003
Recentlyweshowedthatvisible-UVspectrainaqueoussolutioncanbeaccuratelycalculatedforarsenic( )
III
bisul?des,suchasAs(SH)3,As(SH)2S2andtheiroligomers.Thecalculatedlowestenergytransitionsforthese
specieswerediagnosticoftheirprotonationandoligomerizationstat
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