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活化热钾碱吸收CO2动力学.pdf

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活化热钾碱吸收CO2动力学

Hans Journal of Chemical Engineering and Technology 化学工程与技术, 2012, 2, 103-107 doi:10.4236/hjcet.2012.24018 Published Online October 2012 (/journal/hjcet.html) Study on CO Absorption with Aqueous Potassium Carbonate 2 * Solution Promoted by Boric Acid # Shufeng Shen , Xiaoxia Feng Hebei Research Center of Pharmaceutical and Chemical Engineering, School of Chemical and Pharmaceutical Engineering, Hebei University of Science and Technology, Shijiazhuang Email: #shufengshen@ Received: Aug. 8th rd th , 2012; revised: Sep. 3 , 2012; accepted: Sep. 10 , 2012 Abstract: The addition of promoter into aqueous potassium carbonate solution is one of the effective ways to enhance the CO absorption rate. In this work, the CO absorption rates were investigated for aqueous carbonate solution pro- 2 2 moted by different addictives in a wetted wall column. The effect of concentration of boric acid on the overall gas-phase mass transfer coefficient and vapor-liquid equilibrium data was discussed. Results showed that the addition of boric acid can significantly enhance the CO2 absorption rate. The overall mass transfer coefficient increased by 80% with the addition of 3 wt% boric acid. CO2 partial pressure increased with the increasing temperature of aqueous potassium car- bonate. However it decreased when boric acid was added, which would be favorable for CO2 absorption. Keywords: Carbon Dioxide Absorption; Potassium Carbonate; Boric Acid; Vapor-Liquid Equilibrium