测量放射性核素在岩石样品中扩散系数的新方法.pdf

18-P-418 测量放射性核素在岩石样品中扩散系数的新方法 * 冯孝贵 ，梁俊福，王建晨，陈 靖 清华大学核能与新能源技术研究院，北京102201 E-mail:fengxiaogui@tsinghua.edu.cn 放射性核素在处置库围岩中的扩散系数是评价处置库性能的重要参数。文献报道的方法是沿着 核素扩散方向将岩石样品分层磨削逐层测量。由于岩石样品很硬，并且样品含有放射性，因此磨削 操作非常困难。本研究将磷屏放射自显影法与程序计算相结合，测得了 241Am 在花岗岩中的扩散系 数。该方法避免了直接对放射性岩石样品进行磨削的操作，因而比文献方法更加简单易行。 L I 低 ∫ c(x ) ⋅f d (x) ⋅f s (x ) ⋅dx cc==cc((xx)) 0 I L 高 ∫ c(x ) ⋅f d (L − x) ⋅f s (L − x ) ⋅dx 0 xx dxdx LL Fig. 1 Schematic diagram of measurement principle 关键词：扩散系数；放射性核素；岩石；磷屏；放射自显影。 参考文献： [1] Ittner T, Torstenfelt B, Allard B. Radiochimica acta,1988,44/45:171-177. [2] Cole J M, Nienstedt J, Spataro G, et al. Chemical geology, 2003, 193: 127- 136. A new approach to determine the diffusivities of radionulides in rock Xiao-Gui FENG, Jun-Fu LIANG, Jian-Chen WANG, Jing CHEN Institute of Nuclear and New Energy Technology, Tsinghua University, P.O. Box 1021, Beijing 102201 The diffusivities of radionuclides in host rock are important for the performance assessment of repositories. The reported method for determining the diffusivities of radionuclides is to remove successive 0.05-0.1mm thick layers of the rock tablet by grinding and then to measure the activity remaining on the rock tablet before each grinding cycle. Since it is