内应力对用于非致冷红外探测器的Ba068Sr032TiO3-Ba068Sr0322TiO4材料介电和场致热释电性能的影响.docVIP

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内应力对用于非致冷红外探测器的Ba068Sr032TiO3-Ba068Sr0322TiO4材料介电和场致热释电性能的影响.doc

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内应力对用于非致冷红外探测器的Ba068Sr032TiO3-Ba068Sr0322TiO4材料介电和场致热释电性能的影响

Role of internal stress on dielectric and dc bias field-induced pyroelectric properties of Ba0.68Sr0.32TiO3-(Ba0.68Sr0.32)2TiO4 for uncooled 5 10 15 20 25 infrared detectors# ZHANG Guangzu, YI Jinqiao, JIANG Shenglin, YU Yan, HE Jungang, LIU Sisi, ZHU Dingyang, ZHANG Ling** (School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan 430074, China) Abstract: Ba0.68Sr0.32TiO3-(Ba0.68Sr0.32)2TiO4 ceramic were fabricated by the solid-state reaction process, and the microstructural, dielectric, and pyroelectric properties were systemically investigated. In Ba0.68Sr0.32TiO3 ceramics with slight Ba/Sr-excess composition, (Ba0.68Sr0.32)2TiO4 second-phase was found in the center of Ba0.68Sr0.32TiO3 grains and the “core-shell” grain structure was formed. Compared with Ba0.68Sr0.32TiO3 ceramic, Ba0.68Sr0.32TiO3-(Ba0.68Sr0.32)2TiO4 with “core-shell” grain structure exhibited steeper dielectric constant slope, sharper dielectric constant peak and approximately 50% higher dc bias field-induced pyroelectric coefficient. The factors affecting the dielectric and pyroelectric properties anomaly were discussed from a viewpoint of thermal stress effect. The high stress due to the thermal mismatch with the (Ba0.68Sr0.32)2TiO4 second-phases resulted in the change of dielectric properties and the increase of pyroelectric coefficient. The improvement of pyroelectric property would be very useful for the development of BST dielectric bolometer. Key words: BST ceramic; Internal stress; Core-shell grain structure; Dielectric property; Dc bias field-induced pyroelectric property 0 Introduction Barium strontium titanate (BST) is a promising pyroelectric material for infrared detector and thermal imaging[1-6].The pyroelectric coefficient of pyroelectric materials can be expressed as[6]: E 0 Where P0 is the pyroelectric coefficient in the absence of dc bias field, (1) ? 0 is the permittivity in vacuum, ? r is the relative dielectric constant of t