天气条件及气团来源对青岛春季大气颗粒物数浓度谱分布的影响.PDF

中国环境科学 2012,32(8) ：1392~1399 China Environmental Science 天气条件及气团来源对青岛春季大气颗粒物数浓度谱分 布的影响 李瑞芃 1,石金辉 1,2*,张代洲 3 ( 中国海洋大学环境科学与工程学院, 山东 青岛 266100 ；2. 中国海洋大学海洋环境 与生态教育部重点实验室, 山东 青岛 266100 ；3. 日本熊本县立大学环境共生学部, 日 熊 862-8502) 摘要：利用 2010 年春季在青岛观测的不同粒径大气颗粒物数浓度,结合同期的 Micaps 天气图资料及后向轨迹分析资料,探讨了不同天气条 件及气团来源不同时青岛大气颗粒物数浓度谱的变化特征.结果表明,沙尘发生前 12h,大气中 0.3~1.0µm 的细粒子数浓度逐渐小幅升高,沙 尘发生时1.0µm 粗颗粒物数浓度较沙尘发生前升高了 1~10 倍,0.3~1.0µm 细颗粒物数浓度则降低了 20%~45%. 降雨使1.0µm 粗粒子数浓 度降低50%, 降雨后大气颗粒物尤其是细粒子数浓度很快回升.雾和霾天气发生时1.0µm 细粒子数浓度较之雾、霾前均明显升高,雾对 0.7~1.0µm 颗粒物的影响较大,而霾对 0.5~0.7µm 颗粒物的影响较大.气团来源对青岛大气颗粒物数浓度及其谱分布有一定影响,沙尘源气溶 胶中1.0µm 粗粒子数浓度较高,而局地源气溶胶中粗粒子数浓度较低,0.7µm 细粒子相对贡献较大. 关键词：大气颗粒物；数浓度谱；沙尘；霾；雾 中图分类号：X513 文献标识码：A 文章编号：1000-6923(2012)08-1392-08 Size distribution of atmospheric particles in number concentration in relation to meteorological conditions and air 1 1,2* 3 mass origins in Qingdao in spring. LI Rui-peng , SHI Jin-hui , ZHANG Dai-zhou (1.College of Environmental Science and Engineering, Ocean University of China, Qingdao 266100 China；2.Key Laboratory of Marine Environmental Science and Ecology, Ministry of Education, Ocean University of China, Qingdao 266100 China; 3.Faculty of Environmental and Symbiotic Sciences, Prefectural University of Kumamoto, Kumamoto 862-8502, Japan). China Environmental Science, 2012,32(8)：1392~1399 Abstract ：Number concentrations of atmospheric particles were measured in the suburban area of Qingdao in the spring of 2010. Size distributions of number concentrations of atmospheric particles were investigated in terms of impacts of meteorological conditions (e.g., Micaps weather charts and the calculated air mass back trajectories) and various air mass origins. The results showed t