原创力文档removal of hydrophobic organic contaminants from aqueous solutions by sorption onto biodegradable polyesters疏水性有机污染物的去除水溶液的吸附到生物可降解聚酯.pdf
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removal of hydrophobic organic contaminants from aqueous solutions by sorption onto biodegradable polyesters疏水性有机污染物的去除水溶液的吸附到生物可降解聚酯
J. Water Resource and Protection, 2010, 2, 214-221
doi:10.4236/jwarp.2010.23024 Published Online February 2010 (/journal/jwarp)
Removal of Hydrophobic Organic Contaminants from
Aqueous Solutions by Sorption onto
Biodegradable Polyesters
1 1 2
Yukiko Matsuzawa , Zen-Ichiro Kimura , Yoshiro Nishimura ,
Mikio Shibayama2, Akira Hiraishi1*
1
Department of Ecological Engineering, Toyohashi University of Technology, Toyohashi, Japan
2Mikawa Textile Research Institute, Aichi Prefecture, Gamagori, Japan
E-mail : hiraishi@eco.tut.ac.jp
Received November 7, 2009; revised November 24, 2009; accepted January 21, 2010
Abstract
Sorption by biodegradable polyesters of several aromatic chemicals as model compounds for hydrophobic
organic contaminants (HOCs) was studied. The biodegradable polyesters used were poly(butylene succinate),
poly(3-hydroxybutyrate-co-3-hydroxyvalerate), poly(ε-caprolactone), poly(butylene succinate/ terephthalate),
and poly(L-lactic acid). Petrochemical plastics, low-density polyethylene and polyethylene terephtalate, were
used for comparison. The target HOCs were biphenyl, bisphenol-A, dibenzofuran, diethylstilbestrol, nonyl-
phenol, and chlorophenols. The treatment of the HOC solutions with each of the biodegradable polyesters
resulted in the nearly complete removal of the chemicals by sorption from the aqueous phase, except for the
case of poly(L-lactic acid). Low-density polyethylene adsorbed biphenyl and dibenzofuran selectively, and
polyethylene terephtalate did not adsorb any of the HOCs. The adsorptive interaction between the plastics
and the HOCs might be related to both
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