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Hindawi Publishing Corporation Journal of Nanotechnology Volume 2012, Article ID 216050, 10 pages doi:10.1155/2012/216050 Research Article Self-Organization of K+-Crown Ether Derivatives into Double-Columnar Arrays Controlled by Supramolecular Isomers of Hydrogen-Bonded Anionic Biimidazolate Ni Complexes Makoto Tadokoro,1 Kyosuke Isoda,1 Yasuko Tanaka,1 Yuko Kaneko,1 Syoko Yamamoto,1 Tomoaki Sugaya,1 and Kazuhiro Nakasuji2 1 Department of Chemistry, Faculty of Science, Tokyo University of Science, Kagurazaka 1-3, Shinjuku-ku, Tokyo 162-8601, Japan