天津纪庄子污水处理厂恶臭气体排放研究-环境科学研究.docVIP

天津市某社区老年人PM2.5暴露痕量元素健康风险评估 摘要：为研究PM2.5暴露特征，对天津市某社区101名老年人(平均年龄67岁)夏季(2011年6月13日―7月2日)和冬季(2011年11月30日―12月12日)PM2.5暴露水平进行了监测，并分析了PM2.5载带痕量元素含量及其健康风险. 结果表明，研究对象夏、冬季PM2.5个体暴露浓度分别为(124.2±75.2)、(170.8±126.6) μg/m3，室内暴露浓度分别为(120.0±48.9)、(164.9±125.7) μg/m3环境暴露浓度分别为(98.6±33.3)、(140.0±87.7)μg/m310种痕量元素中，ρ(Zn最高，占总浓度%以上；V、Cr、Mn、Cu、Zn和Pb的非致癌风险值均小于1，理论风险较小，；As和总体致癌风险均超过10-6，对于人体的危害不容忽视. 关键词：老年人；PM2.5；痕量元素；风险评估 中图分类号：X55 文献标志码：A 稿件： Health Risk Assessment of Trace Elements of PM2.5 Exposure for the Elderly Subpopulation in Tianjin, China Abstract：To investigate exposure characteristics of PM2.5, a panel study was conducted for elderly subpopulation in Tianjin. A total of 101 elderly participants (mean age 67) were selected and their exposure of PM2.5 were monitored longitudinally in summer (13th June-2nd July) and winter (30th November-12th December) of 2011. Personal and indoor PM2.5 samples were collected by personal environmental sampler. Ambient PM2.5 samples were obtained by median-volume PM2.5 sampler. All the samples were analyzed using inductively coupled plasma-mass spectroscopy (ICP-MS) for trace elements (V, Cr, Mn, Co, Ni, Cu, Zn, As, Cd and Pb). The results showed that the personal, indoor and ambient PM2.5 concentrations were (124.2±75.2) μg/m3, (120.0±48.9) μg/m3, (98.6±33.3) μg/m3 for summer, and (170.8±126.6) μg/m3, (164.9±125.7) μg/m3, (140.0±87.7) μg/m3 for winter, respectively. The result of the concentration analysis of trace elements showed that Zn was the most abundant element, accounting for over 35% of the total trace element concentration. The Hazards Quotient (HQ) of 6 non-cancer-risk elements (V, Cr, Mn, Cu, Zn and Pb) were all below 1. The HQ of Cr and Mn were higher than 0.1, which might have non-cancer-risk for the elderly subpopulation. The median value of Incremental Lifetime Cancer Risk (ILCR) of As was 1.12×10-5. The total ILCR and ILCRs of As and Cd were all higher than the acceptable risk level of 10-6, indicating an unacceptable p