原创力文档titanium dioxide-mediated photcatalysed degradation of two herbicide derivatives chloridazon and metribuzin in aqueous suspensions钛dioxide-mediated photcatalysed退化两种除草剂衍生品chloridazon和赛克津水悬浮液.pdfVIP
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titanium dioxide-mediated photcatalysed degradation of two herbicide derivatives chloridazon and metribuzin in aqueous suspensions钛dioxide-mediated photcatalysed退化两种除草剂衍生品chloridazon和赛克津水悬浮液
Hindawi Publishing Corporation
International Journal of Chemical Engineering
Volume 2012, Article ID 850468, 8 pages
doi:10.1155/2012/850468
Research Article
Titanium Dioxide-Mediated Photcatalysed Degradation of
Two Herbicide Derivatives Chloridazon and Metribuzin in
Aqueous Suspensions
A. Khan,1 N. A. Mir,1 M. Faisal,2 and M. Muneer1
1 Department of Chemistry, Aligarh Muslim University, Aligarh 202002, India
2 Centre of Advanced Materials and Nano-Engineering (CAMNE), Najran University, P.O. Box 1988, Najran 11001, Saudi Arabia
Correspondence should be addressed to M. Muneer, readermuneer@
Received 9 October 2011; Revised 20 February 2012; Accepted 7 March 2012
´
Academic Editor: Licınio M. Gando-Ferreira
Copyright © 2012 A. Khan et al. This is an open access article distributed under the Creative Commons Attribution License, which
permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
The aim of this paper is to find out the optimal degradation condition for two potential environmental pollutants, chloridazon and
metribuzin (herbicide derivatives), employing advanced oxidation process using TiO2 photocatalyst in aqueous suspensions. The
degradation/mineralization of the herbicide was monitored by measuring the change in pollutant concentration and depletion
in TOC content as a function of time. A detailed degradation kinetics was studied under different conditions such as types of
TiO2 (anatase/anatase-rutile mixture), catalyst concentration, herbicide concentration, initial reaction pH, and in the presence of
electron acceptors (hydrogen peroxide, ammonium persulphate, potassium persulphate) in addition to atmospheric oxygen. The
photocatalyst, Degussa P25, was found to be more effi
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