原创力文档a new bedt-ttf-based organic charge transfer salt with a new anionic strong acceptor, n,n-disulfo-1,4-benzoquinonediimine新的bedt-ttf-based有机电荷转移盐阴离子受体,n,n -disulfo-1 4-benzoquinonediimine.pdfVIP
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a new bedt-ttf-based organic charge transfer salt with a new anionic strong acceptor, n,n-disulfo-1,4-benzoquinonediimine新的bedt-ttf-based有机电荷转移盐阴离子受体,n,n -disulfo-1 4-benzoquinonediimine
Crystals 2012, 2, 182-192; doi:10.3390/cryst2020182
OPEN ACCESS
crystals
ISSN 2073-4352
/journal/crystals
Communication
A New BEDT-TTF-Based Organic Charge Transfer Salt with a
New Anionic Strong Acceptor, N,N -Disulfo-1,4-
benzoquinonediimine
Hiroki Akutsu 1,*, Jun-ichi Yamada 1, Shin’ichi Nakatsuji 1 and Scott S. Turner 2
1 Graduate School of Material Science, University of Hyogo, 3-2-1 Kouto, Kamigori-cho, Ako-gun,
Hyogo 678-1297, Japan
2 Department of Chemistry, University of Surrey, Guildford, Surrey, GU2 7XH, UK
* Author to whom correspondence should be addressed; E-Mail: akutsu@sci.u-hyogo.ac.jp;
Tel.: +81-791-58-0164; Fax: +81-791-58-0164.
Received: 21 February 2012; in revised form: 27 March 2012 / Accepted: 28 March 2012 /
Published: 10 April 2012
Abstract: A novel organic dianion, N ,N-Disulfo-1,4-benzoquinonediimine (1) has been
prepared, which is a strong electron acceptor. The reduction potential of the PPh4 salt
indicates that 1 is a stronger acceptor than DDQ (2,3-dichloro-5,6-dicyano-1,4-
benzoquinone). The dianionic acceptor provided a BEDT-TTF salt, (BEDT-TTF) 1·3H O,
4 2
the structures and physical properties of which are reported.
Keywords: organic conductor; BEDT-TTF; hole doping effect; anionic acceptor; transport
properties; magnetic properties
1. Introduction
After the first preparation of bis(ethylenedithio)tetrathiafulvalene (BED
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