spontaneous enhancement of packing regularity of spherical microdomains in the body-centered cubic lattice upon uniaxial stretching of elastomeric triblock copolymers包装球形microdomains规律的自发的增强体心立方晶格在单轴拉伸弹性triblock共聚物.pdfVIP

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spontaneous enhancement of packing regularity of spherical microdomains in the body-centered cubic lattice upon uniaxial stretching of elastomeric triblock copolymers包装球形microdomains规律的自发的增强体心立方晶格在单轴拉伸弹性triblock共聚物.pdf

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spontaneous enhancement of packing regularity of spherical microdomains in the body-centered cubic lattice upon uniaxial stretching of elastomeric triblock copolymers包装球形microdomains规律的自发的增强体心立方晶格在单轴拉伸弹性triblock共聚物

Polymers 2011, 3, 36-50; doi:10.3390/polym3010036 OPEN ACCESS polymers ISSN 2073-4360 /journal/polymers Article Spontaneous Enhancement of Packing Regularity of Spherical Microdomains in the Body-Centered Cubic Lattice upon Uniaxial Stretching of Elastomeric Triblock Copolymers Takuya Kota 1, Kimio Imaizumi 2, Sono Sasaki 1 and Shinichi Sakurai 1,3,* 1 Department of Biobased Materials Science, Graduate School of Science and Technology, Kyoto Institute of Technology, Matsugasaki, Sakyo-ku, Kyoto 606-8585, Japan; E-Mail: sono@kit.ac.jp 2 Asahi-kasei Corporation, 1-1-2 Yurakucho, Chiyoda-ku, Tokyo 100-8440, Japan; E-Mail: imaizumi.kc@om.asahi-kasei.co.jp 3 Center for Fiber and Textile Science, Kyoto Institute of Technology, Matsugasaki, Sakyo-ku, Kyoto 606-8585, Japan * Author to whom correspondence should be addressed; E-Mail: shin@kit.ac.jp; Tel.: +81-75-724-7864; Fax: +81-75-724-7800. Received: 26 October 2010; in revised form: 14 December 2010 / Accepted: 22 December 2010 / Published: 2 7 December 2010 Abstract: Block copolymers forming glassy spheres in the matrix of rubbery chains can exhibit elastomeric properties. It is well known that the spherical microdomains are arranged in the body-center cubic (bcc) lattice. However, recently, we have found packing in the face-centered cubic (fcc) lattice, which is easily transformed into the bcc lattice upon uniaxial stretching. In the same time, the packing regularity of the spheres in the bcc lattice was found to be enhanced for samples completely recovered from the stre