模拟烟气中硅灰石矿物碳酸化隔离CO2的试验研究.PDF

第30 卷 第11 期 中 国 电 机 工 程 学 报 Vol.30 No.11 Apr.15, 2010 44 2010 年4 月15 日 Proceedings of the CSEE ©2010 Chin.Soc.for Elec.Eng. 0258-8013 (2010) 11-0044-06 X 701 A 470 10 文章编号： 中图分类号： 文献标志码： 学科分类号： ⋅ 模拟烟气中硅灰石矿物碳酸化隔离CO 的实验研究 2 晏恒，张军营，王志亮，赵永椿，郑楚光 (煤燃烧国家重点实验室(华中科技大学) ，湖北省 武汉市 430074) Carbon Dioxide Sequestration by Mineral Carbonation in Simulated Flue Gas Using Wollastonite YAN Heng, ZHANG Jun-ying, WANG Zhi-liang, ZHAO Yong-chun, ZHENG Chu-guang (State Key Laboratory of Coal Combustion (Huazhong University of Science and Technology), Wuhan 430074, Hubei Province, China) ABSTRACT: Wollastonite was used as the mineral raw 6 MPa ，硅灰石碳酸化转化率从 18.7%增加到 28.8% ；SO2 material for carbon dioxide sequestration as direct mineral 的存在不利于较高温度下硅灰石矿物碳酸化固定CO ，平均 2 carbonation in the simulated flue gas, and experiments were 降低5%；在模拟烟气条件下，4 MPa 、200 ℃时反应60 min carried out to review the effects of temperature, pressure and 得到最高矿物碳酸化效率为30.2% 。 the addition of SO2 on the carbonated efficiency. The 关键词：CO ；模拟烟气；矿物碳酸化；硅灰石；隔离 2 experiment results show that the carbon dioxide can be directly sequestrated as carbonate using wollastonite under a 0 引言 certain temperature and pressure conditions in simulated flue 我国能源的供给约70%