原创力文档dynamic nuclear polarization via thermal mixing beyond the high temperature approximation：（动态核极化通过热混合在高温近似）.pdfVIP
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dynamic nuclear polarization via thermal mixing beyond the high temperature approximation：（动态核极化通过热混合在高温近似）
Journal of Magnetic Resonance 277 (2017) 68–78
Contents lists available at ScienceDirect
Journal of Magnetic Resonance
journal homepage: www.else /locate/jmr
Dynamic nuclear polarization via thermal mixing: Beyond the high
temperature approximation
W.Th. Wenckebach
Paul Scherrer Institute, CH-5232 Villigen, Switzerland
a r t i c l e i n f o a b s t r a c t
Article history: Dynamic Nuclear Polarization (DNP) via the mechanism of thermal mixing has proven itself most pow-
Received 13 December 2016 erful for the orientation of nuclear spins in polarized targets and hyperpolarization for magnetic reso-
Revised 26 January 2017 nance imaging (MRI). Unfortunately, theoretical descriptions of this mechanism have been limited to
Accepted 29 January 2017
using—at least partially—the high temperature approximation, in which Boltzmann factors are expanded
Available online 20 February 2017
linearly. However, the high nuclear spin polarization required and obtained for these applications does
not justify such approximations.
Keywords:
This article extends the description of thermal mixing beyond the high temperature approximation, so
Dynamic nuclear polarization
Boltzmann factors are not expanded. It applies for DNP in samples doped with paramagnetic centres, for
Hyperpolarization
Thermal mixing
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