表面等离子体增强有机发光二极管的研究-凝聚太物理专业论文 word格式.docxVIP

AbstractStudies of Surface Plasmon-Polariton Enhanced Organic Light-Emitting DiodeStudies of Surface Plasmon-Polariton Enhanced Organic Light-Emitting DiodesAbstractOrganic light-emitting diodes (OLEDs) have drawn a lot of attention in flat panel display and solid-state lighting due to their advantages such as low power consumption, high brightness and full color. High efficient OLEDs are mainly limited by two factors: one is the internal quantum efficiency (IQE) of OLEDs, the other is the out-coupling efficiency of OLEDs.Surface plasmon-polariton (SPP) is the electromagnetic wave localized at the interface between the metal and dielectric material. As it has many novel properties, such as enhancing the spontaneous emissive rate of nearby fluorescent molecules and coupling with photons in specific structures, SPP is widely studied in many emerging areas. Moreover, there is about 40% of the total energy lost in the SPP mode for the traditional OLEDs.Accordingly, the following two systems of surface plasmon- polariton effects are studied in OLEDs and their mechanisms are also investigated in the thesis.Firstly, we inserted silver nano-particles in different positions in OLEDs and studied their influences on the efficiency. We found that the energy could be transferred between excitons and SPPs. With a suitable separation distance, the current efficiency of OLED can be enhanced as much as 20%. In addition, we demonstrated that the energy transfer is affected not only by the distance between nano-particles and the emissive layer, but also by the distance between nano-particles and the metallic cathode.Secondly, we fabricated the OLED devices with a 2D quasi-periodic array structure based on the monolayer colloidal crystal of polystyrene spheres. The lost energy due to SPP mode is effectively extracted. The device current efficiency at 40 mA/cm2 is enhanced by 27.7% and the intensity of electroluminescent (EL) spectrum is improved by 60% at 600 nm. Furthermore, we confi