卤氧化铋半导体材料的表面结构调控及其光催化性能分析-surface structure control and photocatalytic performance analysis of bismuth oxyhalide semiconductor materials.docxVIP

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卤氧化铋半导体材料的表面结构调控及其光催化性能分析-surface structure control and photocatalytic performance analysis of bismuth oxyhalide semiconductor materials.docx

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卤氧化铋半导体材料的表面结构调控及其光催化性能分析-surface structure control and photocatalytic performance analysis of bismuth oxyhalide semiconductor materials

卤氧化卤氧化铋半导体材料的表面结构调控及其光催化性能研究摘要 PAGE PAGE IVStudy of surface structure modulation and photocatalytic property of bismuth oxyhalides semiconductor materialsBenyan Xu (Physical chemistry)Abstract: Photocatalytic technology has attracted wordwide attention due to its potential applications in solving the problems of energy shortage and environment pollution. Compared with the traditional treatments, photocatalytic materials could thoroughly decompose organic pollutants to CO2 and H2O, and show many merits of low cost, high photocatalytic efficiency, less secondary pollution and so on. However, from the viewpoint of efficient utilization of solar energy, seeking novel photocatalysts with high photocatalytic activity under visible light is an inevitable trend for the further practical application of photocatalytic technology. Recently, bismuth oxyhalides (BiOX, X =Br, I) with good light absorption and photochemical stability have become the hot topics in the research of novel photocatalytic materials. Thus, the purpose of this thesis is to build a new type of BiOX/semiconductor (BiOX/SC) heterojunction photocatalysts with high photocatalytic activity through band matching and structure tuning. Meanwhile, the separation process of photogenerated electron-hole pairs and the detection process of reactive species were also discussed to provide a reasonable mechanism for the enhanced photocatalytic activity.The main research contents and important results of this thesis are presented as follows:BiOI/BiOBr heterojunction photocatalyst was prepared by a modified deposition-precipitation method and characterized by XRD、SEM、HRTEM、BET、DRS. Methyl orange (MO) was selected as a polutant model to evaluated the visible-lightphotocatalytic acticity of BiOI/BiOBr. The results showed that BiOI/BiOBr exhibited higher photocatalytic activity than single BiOI and BiOBr. BiOI-BiOBr heterojunction formed in BiOI/BiOBr was a key factor for the enhanced photocatalytic activity. Moreover, ?O2?