湿法脱硫后烟气细颗粒物的声团聚1.docVIP

硕士学位论文 湿法脱硫后烟气细颗粒物的声波团聚 ACOUSTIC AGGLOMERATION OF FINE PARTICLES FROM WFGD 摘 要 随着我国能源消耗量的逐渐增加，细颗粒物的污染已成为不容忽视的环境问题。燃煤烟气产生的颗粒物是我国空气中细颗粒物的主要来源之一，而传统烟气除尘装置对细颗粒物脱除效率很低。烟气经过湿法脱硫系统后将形成由脱硫产物包裹的细颗粒物，难以通过传统除尘装置脱除。因此，本文对脱硫后烟气中的细颗粒物在声波作用下的团聚现象进行了数值模拟研究。 选择同向团聚和流体力学作用作为声团聚室中颗粒团聚的主要团聚机理。在这两种主要团聚机理的团聚核函数基础上，添加布朗团聚核函数，以提高模拟结果的准确性。数值模拟采用在电厂现场测试获得的脱硫后烟气颗粒物粒径分布的实际数据为初始条件，颗粒物粒径分布范围取为0.2~10μm。对传统分组算法进行改进，使其可根据细颗粒物质量浓度分布自动调整分组的大小，以提高计算精度。计算结果显示，提高声波频率对提高颗粒数目减少率的效果不明显，而提高声强级能显著提高颗粒数目减少率，高声强级更适于脱硫后烟气中颗粒物的团聚。综合考虑经济性和颗粒质量浓度分布，对于每一种颗粒物粒径分布，应选用不同声波频率和声强级的声波。 借鉴旋风分离器的结构，提出了一种旋风式声团聚室，以提高颗粒物在声团聚室中的停留时间，从而提高声波团聚的效率。采用欧拉-拉格朗日方法进行数值模拟的结果显示，进口速度为12m/s时，1μm的颗粒物在旋风式声团聚室中的停留时间为1.2s。 耦合欧拉多流体模型和颗粒群平衡模型对声团聚室进行了数值模拟研究。主要分析了不同条件下，旋风式声团聚室出口颗粒数目浓度减少量的变化规律和其产生的压力损失。模拟结果显示，旋风式声团聚室出口颗粒数目浓度的减少量随声波频率和声强级的增加而增加；烟气流速与烟气处理量和团聚效果有关；旋风式声团聚室产生的压力损失较小，因此对尾部烟气系统的影响也较小。 关键词：声波团聚；脱硫后烟气；分组算法；细颗粒物；数值模拟 Abstract As China’s energy consumption continue increasing, pollution problem rised by fine particles is becoming a serious environmental problem. Particles from flue gas make an important contribution to fine particle pollution in China. It is difficult to remove fine particles effectively by conventional dust remover. Fine particles enwrapped with desulfurization reaction products will be formed after the wet flue gas desulfurization (WFGD). Numerical simulation of coagulation fine particles from the WFGD in acoustic field has been studied in this thesis. Orthokinetic and hydrodynamic are chosen as coagulation mechanism based on the existing acoustic agglomeration model in this study. Brownian coagulation kernel has also been considered simultaneously for accuracy of the computation. The initial particle size distribution of the numerical computation is confirmed between 0.2μm and 10μm, which is based on experimental measurement data of flue gas after the WFGD from plant station. Sectional arithmetic is developed to improve computation precision. With the developed sectional arithmetic, group size is connected to particle ma