毕业论文毕业设计格式（完整）.doc

XX大学毕业论文 (学校图标) #### 届毕业（设计）论文 (学校名称) 题 目 专业班级 学 号 学生姓名 指导教师 指导教师职称 学院名称 完成日期： 年 月 日 毕业设计（论文）题目及副标题（中文） 毕业设计（论文）题目及副标题（英文） 学生姓名 指导教师 摘 要（黑体，四号，居中） XXXX是一种对环境友好的绿色化学品，其洁净合成工艺的研究及开发，已引起国内外学者的广泛关注。以XXXX催化剂甲醇液相氧化羰化法合成XXXX已实现工业化。由于反应生成了副产物XXXX，造成XXXX的流失，不仅造成催化剂失活，同时对反应设备腐蚀严重，污染环境。 论文中制备了XXXX均相催化剂，并采用IR对其进行了表征。考察了不同XXXX对XXXX催化性能的影响。结果表明：XXXX制备的催化剂催化活性最高。在120℃，反应压力2.4MPa，反应时间4h条件下，xxxx的转化率达到5.8%，DMC的选择性达到99.9%。对于双配体络合XXXX催化体系，能进一步提高催化活性。在120℃，反应压力2.4MPa，反应时间Xh，XXXX：N-甲基咪唑：XXXX=2：1：1 (摩尔比)，XXXX的转化率达到6.6%。结果同时表明，催化体系的XXXX的流失量降低，催化剂的寿命得到了提高。 关键词：XXXX；XXX；XXX  Abstract（黑体，四号，居中） Diethyl carbonate (DMC) is an environmentally benign intermediation. It was paid widely attention that the research and development of a green process of synthesis of DMC. Although the process of producing DMC by oxidative carbonization of methanol in the presence of CuCl catalyst system has been industrial, some drawbacks, for instance the production of the by-production HCl , in which not only caused to a leaking of Cl- subsequence by the deactivate of the catalyst, but also a corrosion to the reactor, still need to be overcome. In this work, a complex catalyst was prepared from CuCl and Schiff base additives and characterized by IR. The effects of different Schiff base additives were investigated. The results showed that high activity was exhibited in the presence of complex catalyst synthesized by N-methylimidazole and CuCl，the methanol conversion was 5. 8%, DMC selectivity reached to 99.9 % at 120 ℃, pressure 2.4 MPa, the reaction time 4 h. At the same condition, catalytic activity was further improved by t