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2008,28(12) 1084~1087 China Environmental Science
2
*
,, , (, 310032)
γAl O /SnO +Sb O 2(2CP),pH ,
2 3 2 2 4
.,2CP ,90min ,2CP TOC 97.0%58.9%.
,(15 min),, 1.7 .LCMS IC ,2CP
()(),.
2
X703.1 A 2008
*
Decomposition of 2-chlorophenol by three-phase fluidized bed. ZHU Run-ye, PAN Wei-wei, WANG Jia-de , CHEN
Jian-meng (Research Center of Environmental Engineering, Zhejiang University of Technology, Hangzhou 310032,
China). China Environmental Science, 2008,28(12)1084~1087
Abstract Decomposition of 2-chlorophenol (2CP) by three-phase fluidized bed packed with γAl O /SnO +Sb O as
2 3 2 2 4
particle electrode was investigated. The effect of pH values and particle electrode on 2CP removal efficiency were
determined. The removal efficiency of 2CP and TOC reached about 97.0% and 58.9% after 90min under alkaline
condition, which was higher than that under acidity or neutral condition. Particle electrode was beneficial to increase the
current efficiency. The current efficiency of three-phase fluidized bed was 1.7 times higher than that of the conventional
structure with no particle electrode at 15min. The analysis results from LC-MS and IC indicated that CC double bonds in
benzene ring of 2CP was broken first, and formed some intermediate products, such as 2Clp(o)hydroquinone,
2Clp(o)benzoquinone, succinic acid, acetic acid, formic acid and so on.
Key words three-phase fluidized bed particle electrode 2chlorophenol
, Ti/SnO +Sb O
2 2 4
, 2.5cm. γ Al O /
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