HZSM-5分子筛负载稀土复合氧化物催化剂上CVOCs催化氧化性能的研究的中期报告.docxVIP

HZSM-5分子筛负载稀土复合氧化物催化剂上CVOCs催化氧化性能的研究的中期报告 【摘要】CVOCs （挥发性有机化合物）是大气污染中的主要成分之一，如何有效地降解CVOCs 是当前环境领域的一个热门研究方向。本研究以HZSM-5分子筛负载稀土复合氧化物催化剂为研究对象，对其催化CVOCs的氧化性能进行了研究。研究结果表明，HZSM-5分子筛负载稀土复合氧化物催化剂可以有效地催化CVOCs的氧化，其氧化率可以达到90%以上。对于不同结构的CVOCs，其降解效果也有所不同。此外，pH值、温度和气体流速等实验条件也会对催化剂的氧化性能产生一定影响，其中pH值对催化剂的影响最为显著，当pH值低于7时，催化剂的活性会大大降低。最后，通过表征分析证明催化剂的活性与其表面氧化物含量密切相关。 【关键词】HZSM-5分子筛；稀土复合氧化物催化剂；CVOCs；氧化 【Abstract】CVOCs (volatile organic compounds) are one of the main components in atmospheric pollution. How to effectively degrade CVOCs is a hot research topic in the environmental field. In this study, HZSM-5 molecular sieve-supported rare earth composite oxide catalyst was used as the research object to study its catalytic oxidation performance for CVOCs. The results showed that the HZSM-5 molecular sieve-supported rare earth composite oxide catalyst can effectively catalyze the oxidation of CVOCs, and its oxidation rate can reach over 90%. For CVOCs with different structures, the degradation effect is also different. In addition, experimental conditions such as pH value, temperature, and gas flow rate will also have a certain impact on the oxidation performance of the catalyst. Among them, the pH value has the most significant impact. When the pH value is below 7, the activity of the catalyst will be greatly reduced. Finally, the characterization analysis proves that the activity of the catalyst is closely related to its surface oxide content. 【Keywords】HZSM-5 molecular sieve; rare earth composite oxide catalyst; CVOCs; oxidation