磷酸盐系列内容.doc

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Severalolefiniccompoundssuchasvinylacetate,divinyladipateandallylmethylcarbonatewerestudiedasadditivesforpropylenecarbonate

(PC)-basedelectrolytesinlithium-ionbattery,whichkindofelectrolytesalwaysexfoliategraphiticcarbonanddecomposedrasticallytoliberate

organicgas.Threekindsofgraphiticcarbonscommonlyusedinlithium-ionbatteries,namely,naturalgraphite,MCMB6-28andMCFwere

chosentotestthedecomposition-suppressingabilityofadditives.Theeffectsofthetypeofgraphiticanodesandthestructureofadditivesonthe

electrolytedecompositionhavebeeninvestigatedinthetermssolidelectrolyteinterface(SEI)formation,whichwascharacterizedbycyclic

voltammetry(CV),acimpedance,SEM,XPSanalyses,andaugerelectronspectroscopy(AES).Theelectrochemicalperformanceofthe

additives-containingelectrolytesincombinationwithLiCoO2cathodeandgraphiticcarbonanodewasalsotestedincoincells.

Theelectrochemicalperformanceofthermal-vapor-decompositioncarbon-coatednaturalgraphitewasstudiedinbothpropylene

carbonate(PC)-basedelectrolytesandethylenecarbonate(EC)-basedelectrolytes.Inthecyclicvotammogramsofcarbon-coatednatural

graphite,thehumpintherangeof1.3±0.7VversusLi/Licanbeobservedwhenthepotentialwassweptathigherscanrates.Thishump

wasinvestigatedwithreferenceofcarbonblack.Theeffectofelectrode-fabricationpressureontheelectrochemicalperformanceofcarboncoated

inthePC-basedelectrolytehasalsobeenstudied.

Theeffectofcationontheperformanceofactivatedcarbon(AC)/graphitecapacitorhasbeenstudied.ElectrolytesusingLi+andfour

kindsofquaternaryalkylammoniumcationshavebeenpickedupforthisinvestigation.Therelationshipbetweentheionicradiiofcations

andthespecificcapacitanceofACnegativeelectrodeincorrespondingelectrolyteshasbeencorrelated.ThestateofLi+dissolvedin

PC(propylenecarbonate)solventh

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